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100 1 _ |a Krönlein, Andreas
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245 _ _ |a Magnetic Ground State Stabilized by Three-Site Interactions: Fe / Rh ( 111 )
260 _ _ |a College Park, Md.
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520 _ _ |a We report the direct observation of a theoretically predicted magnetic ground state in a monolayer Fe on Rh(111), which is referred to as an up-up-down-down (↑↑↓↓) double-row-wise antiferromagnetic spin structure, using spin-polarized scanning tunneling microscopy. This exotic phase, which exists in three orientational domains, is revealed by experiments with magnetic probe tips performed in external magnetic fields. It is shown that a hitherto unconsidered four-spin–three-site beyond-Heisenberg interaction distinctly contributes to the spin coupling of atoms with S≥1 spins. The observation of the ↑↑↓↓ order substantiates the presence of higher-order, in particular, three-site interactions, in thin magnetic films of itinerant magnets.
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700 1 _ |a Kemmer, Jeannette
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700 1 _ |a Seubert, Nicolai
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700 1 _ |a Vogt, Matthias
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700 1 _ |a Küspert, Julia
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700 1 _ |a Böhme, Markus
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700 1 _ |a Alonazi, Bandar
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700 1 _ |a Kügel, Jens
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700 1 _ |a Albrithen, Hamad A.
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700 1 _ |a Bode, Matthias
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700 1 _ |a Bihlmayer, Gustav
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700 1 _ |a Blügel, Stefan
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773 _ _ |a 10.1103/PhysRevLett.120.207202
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