000848178 001__ 848178
000848178 005__ 20240712084500.0
000848178 0247_ $$2Handle$$a2128/18890
000848178 0247_ $$2URN$$aurn:nbn:de:0001-2018061518
000848178 0247_ $$2ISSN$$a1866-1793
000848178 020__ $$a978-3-95806-329-7
000848178 037__ $$aFZJ-2018-03444
000848178 041__ $$aEnglish
000848178 1001_ $$0P:(DE-Juel1)156496$$aCadiz Bedini, Andrew Paolo$$b0$$eCorresponding author$$gmale$$ufzj
000848178 245__ $$aSonochemical Synthesis of Silicon Hydride Polymers and Silicon Nanoparticles from Liquid Silanes$$f- 2017-12-15
000848178 260__ $$aJülich$$bForschungszentrum Jülich GmbH Zentralbibliothek, Verlag$$c2018
000848178 300__ $$aviii, 132, XVIII S.
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000848178 3367_ $$2ORCID$$aDISSERTATION
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000848178 3367_ $$02$$2EndNote$$aThesis
000848178 3367_ $$0PUB:(DE-HGF)11$$2PUB:(DE-HGF)$$aDissertation / PhD Thesis$$bphd$$mphd$$s1528805659_23107
000848178 3367_ $$2DRIVER$$adoctoralThesis
000848178 4900_ $$aSchriften des Forschungszentrums Jülich Reihe Energie & Umwelt / Energy & Environment$$v423
000848178 502__ $$aRWTH Aachen, Diss., 2018$$bDissertation$$cRWTH Aachen$$d2018
000848178 520__ $$aThe present thesis is concerned with the use of ultrasound for the treatment of liquid silanes with the objective of fabricating solution-processable inks containing silicon hydride polymers and silicon nanoparticles. Also demonstrated is the subsequent use of the inks to deposit semiconducting hydrogenated amorphous silicon(a-Si:H) thin films and for fabricating passivation layers and thin-film photovoltaicdevices.The sonochemical effects of ultrasound on two lower silanes, namely cyclopentasilane(Si5H10) and trisilane (Si3H8) were studied. The processing of the silanes wascarried out in the inert N2-atmosphere and in solution using cyclooctane (C8H16)as solvent at ambient pressure, and at temperatures between -15–70 $^{\circ}$C. Using cyclopentasilane as monomer molecule it was shown via size exclusion chromatography and optical transmission measurements that sonication of 8–15 wt% solutions results in ring-opening polymerization without the need to use ultraviolet light. In addition, through comparisons to purely thermally treated solutions it was demonstrated that the polymerization process is not initiated pyrolytically due to the “macroscopic” temperature of the solution itself, but rather that microscopic effects associated with acoustic cavitation are most likely responsible for triggering polymer growth. [...]
000848178 536__ $$0G:(DE-HGF)POF3-121$$a121 - Solar cells of the next generation (POF3-121)$$cPOF3-121$$fPOF III$$x0
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000848178 9141_ $$y2018
000848178 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)156496$$aForschungszentrum Jülich$$b0$$kFZJ
000848178 9131_ $$0G:(DE-HGF)POF3-121$$1G:(DE-HGF)POF3-120$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lErneuerbare Energien$$vSolar cells of the next generation$$x0
000848178 920__ $$lyes
000848178 9201_ $$0I:(DE-Juel1)IEK-5-20101013$$kIEK-5$$lPhotovoltaik$$x0
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