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@ARTICLE{Nonemacher:848259,
      author       = {Nonemacher, Juliane Franciele and Hüter, Claas and Zheng,
                      Hao and Malzbender, Jürgen and Krüger, Manja and
                      Spatschek, Robert and Finsterbusch, Martin},
      title        = {{M}icrostructure and properties investigation of garnet
                      structured {L}i7{L}a3{Z}r2{O}12 as electrolyte for
                      all-solid-state batteries},
      journal      = {Solid state ionics},
      volume       = {321},
      issn         = {0167-2738},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier Science},
      reportid     = {FZJ-2018-03521},
      pages        = {126 - 134},
      year         = {2018},
      abstract     = {Garnet structured Li7La3Zr2O12 is investigated in its pure,
                      tetragonal phase and its stabilized cubic phase by
                      substitution with different amounts of Ta and Al. The effect
                      of substitution and sintering conditions on phase
                      composition, microstructure, electrical properties and, as
                      main focus, the mechanical properties are investigated.
                      Sintering is carried out in air and argon atmosphere at
                      temperatures of 1150 and 1200 °C. The Ta substitution
                      ranges up to $60\%$ and the Al substitution up to $36\%$ to
                      obtain fully cubic samples. The mechanical properties were
                      assessed via depth-sensitive indentation testing and
                      interpreted in terms of properties of the material and
                      effective properties of the porous specimens. Complementary,
                      ab initio calculations were performed to determine the
                      structural and mechanical properties. The study verifies the
                      strong dependency of the ionic conductivity on substitution,
                      phase composition and materials density. Overall, the effect
                      of substitution and phase composition can be mostly seen in
                      changes in the intrinsic materials properties, whereas the
                      effects of sintering conditions and porosity can mostly be
                      seen in the change in effective mechanical properties.},
      cin          = {IEK-2 / IEK-1 / JARA-HPC},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-2-20101013 / I:(DE-Juel1)IEK-1-20101013 /
                      $I:(DE-82)080012_20140620$},
      pnm          = {111 - Efficient and Flexible Power Plants (POF3-111) / Ab
                      initio modelling of electrode materials for sodium ion
                      batteries $(jiek27_20161101)$ / 1221 - Fundamentals and
                      Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF3-111 / $G:(DE-Juel1)jiek27_20161101$ /
                      G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000437372200019},
      doi          = {10.1016/j.ssi.2018.04.016},
      url          = {https://juser.fz-juelich.de/record/848259},
}