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000850200 1001_ $$0P:(DE-HGF)0$$aJuluri, R. R.$$b0
000850200 245__ $$aCoherently Embedded Ag Nanostructures in Si: 3D Imaging and their application to SERS
000850200 260__ $$aLondon$$bNature Publishing Group$$c2014
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000850200 520__ $$aSurface enhanced Raman spectroscopy (SERS) has been established as a powerful tool to detect very low-concentration bio-molecules. One of the challenging problems is to have reliable and robust SERS substrate. Here, we report on a simple method to grow coherently embedded (endotaxial) silver nanostructures in silicon substrates, analyze their three-dimensional shape by scanning transmission electron microscopy tomography and demonstrate their use as a highly reproducible and stable substrate for SERS measurements. Bi-layers consisting of Ag and GeOx thin films were grown on native oxide covered silicon substrate using a physical vapor deposition method. Followed by annealing at 800°C under ambient conditions, this resulted in the formation of endotaxial Ag nanostructures of specific shape depending upon the substrate orientation. These structures are utilized for detection of Crystal Violet molecules of 5 × 10−10 M concentrations. These are expected to be one of the highly robust, reusable and novel substrates for single molecule detection.
000850200 536__ $$0G:(DE-HGF)POF3-143$$a143 - Controlling Configuration-Based Phenomena (POF3-143)$$cPOF3-143$$fPOF III$$x0
000850200 7001_ $$0P:(DE-HGF)0$$aRath, A.$$b1
000850200 7001_ $$0P:(DE-HGF)0$$aGhosh, A.$$b2
000850200 7001_ $$0P:(DE-HGF)0$$aBhukta, A.$$b3
000850200 7001_ $$0P:(DE-HGF)0$$aSathyavathi, R.$$b4
000850200 7001_ $$0P:(DE-HGF)0$$aNarayana Rao, D.$$b5
000850200 7001_ $$0P:(DE-Juel1)165314$$aMüller-Caspary, Knut$$b6$$ufzj
000850200 7001_ $$0P:(DE-HGF)0$$aSchowalter, Marco$$b7
000850200 7001_ $$0P:(DE-HGF)0$$aFrank, Kristian$$b8
000850200 7001_ $$0P:(DE-HGF)0$$aGrieb, Tim$$b9
000850200 7001_ $$0P:(DE-Juel1)174034$$aKrause, Florian$$b10
000850200 7001_ $$0P:(DE-HGF)0$$aRosenauer, Andreas$$b11
000850200 7001_ $$0P:(DE-HGF)0$$aSatyam, Parlapalli Vencata$$b12$$eCorresponding author
000850200 773__ $$0PERI:(DE-600)2615211-3$$a10.1038/srep04633$$p4633$$tScientific reports$$v4$$x2045-2322$$y2014
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