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@ARTICLE{Gellert:850871,
author = {Gellert, Michael and Dashjav, Enkhetsetseg and Grüner,
Daniel and Ma, Qianli and Tietz, Frank},
title = {{C}ompatibility study of oxide and olivine cathode
materials with lithium aluminum titanium phosphate},
journal = {Ionics},
volume = {24},
number = {4},
issn = {1862-0760},
address = {Berlin},
publisher = {Springer},
reportid = {FZJ-2018-04622},
pages = {1001 - 1006},
year = {2018},
abstract = {The compatibility of the solid electrolyte
Li1.5Al0.5Ti1.5(PO4)3 (LATP) with the cathode materials
LiCoO2, LiMn2O4, LiCoPO4, LiFePO4, and LiMn0.5Fe0.5PO4 was
investigated in a co-sintering study. Mixtures of LATP and
the different cathode materials were sintered at various
temperatures and subsequently analyzed by thermal analysis,
X-ray diffraction, and electron microscopy. Oxide cathode
materials display a rapid decomposition reaction with the
electrolyte material even at temperatures as low as 500 °C,
while olivine cathode materials are much more stable. The
oxide cathode materials tend to decompose to lithium-free
compounds, leaving lithium to form Li3PO4 and other metal
phosphates. In contrast, the olivine cathode materials
decompose to mixed phosphates, which can, in part, still be
electrochemically active. Among the olivine cathode
materials, LiFePO4 demonstrated the most promising results.
No secondary phases were detected by X-ray diffraction after
sintering a LATP/LiFePO4 mixture at temperatures as high as
700 °C. Electron microscopy revealed a small secondary
phase probably consisting of Li2FeTi(PO4)3, which is
ionically conductive and should be electrochemically active
as well.},
cin = {IEK-1 / IEK-12 / IEK-2},
ddc = {530},
cid = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-12-20141217 /
I:(DE-Juel1)IEK-2-20101013},
pnm = {131 - Electrochemical Storage (POF3-131) / SOFC - Solid
Oxide Fuel Cell (SOFC-20140602)},
pid = {G:(DE-HGF)POF3-131 / G:(DE-Juel1)SOFC-20140602},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000428070800005},
doi = {10.1007/s11581-017-2276-6},
url = {https://juser.fz-juelich.de/record/850871},
}