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@ARTICLE{Dagger:851139,
      author       = {Dagger, Tim and Grützke, Martin and Reichert, Matthias and
                      Haetge, Jan and Nowak, Sascha and Winter, Martin and
                      Schappacher, Falko M.},
      title        = {{I}nvestigation of lithium ion battery electrolytes
                      containing flame retardants in combination with the film
                      forming electrolyte additives vinylene carbonate, vinyl
                      ethylene carbonate and fluoroethylene carbonate},
      journal      = {Journal of power sources},
      volume       = {372},
      issn         = {0378-7753},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2018-04841},
      pages        = {276 - 285},
      year         = {2017},
      abstract     = {In order to address the trade-off between the safety
                      lithium ion battery (LIB) electrolytes and their
                      electrochemical performance, synergetic effects of flame
                      retardant additives (FRs) in combination with film forming
                      additives (FFAs) are investigated. Triphenyl phosphate (TPP)
                      and a silicon-containing additive (WA) are applied as FRs to
                      improve the onset temperature of the thermal runaway of a
                      LIB standard electrolyte (LP57: 1 M LiPF6 in EC:EMC 3:7)
                      about 15 K and 28 K, respectively. The application of the
                      FRs in MCMB graphite/lithium metal and NMC111/lithium metal
                      three-electrode cells induces insufficiencies in terms of
                      charge/discharge cycling stability and rate capability.It is
                      investigated if the addition of FFAs can degrade the
                      insufficiencies that are induced by the FRs. Vinylene
                      carbonate, vinyl ethylene carbonate and fluoroethylene
                      carbonate are added to a mixture of LP57 with $10\%$ FR to
                      enhance the cycling performance via improved interphase
                      formation. Results reveal, that the rate capability of cells
                      containing TPP or WA is especially improved by addition of
                      $2\%$ or $5\%$ FEC, respectively.Postmortem analyses of the
                      electrodes by SEM and of the electrolyte by GC-MS are
                      performed. Direct correlations between the cycling behavior
                      during the C-rate study and the electrolyte decomposition
                      products are drawn.},
      cin          = {IEK-12},
      ddc          = {620},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000418392100033},
      doi          = {10.1016/j.jpowsour.2017.10.058},
      url          = {https://juser.fz-juelich.de/record/851139},
}