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000851197 245__ $$aA propylene carbonate based gel polymer electrolyte for extended cycle life and improved safety performance of lithium ion batteries
000851197 260__ $$aNew York, NY [u.a.]$$bElsevier$$c2018
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000851197 520__ $$aA poly(vinylidene difluoride-co-hexafluoropropylene) (PVdF-HFP)-based gel polymer electrolyte (GPE) containing propylene carbonate (PC)-based liquid electrolyte was developed to enhance the safety performance of LiNi0.5Mn0.3Co0.2O2/graphite (NMC532/graphite) lithium ion batteries. The PC-based liquid electrolyte (PEV-LE) consists of 1 mol L−1 LiPF6 as lithium salt, PC as the main solvent and ethylene sulfite (ES, 2% by weight) as well as vinylene carbonate (VC, 2% by weight) as solid electrolyte interphase (SEI) forming additives. Electrochemical impedance spectroscopy (EIS) and X-ray photoelectron spectroscopy (XPS) revealed that the combination of ES and VC additives facilitates the formation of effective interphases at the respective electrolyte/electrode interfaces, thus contributing to a remarkable cycle life of NMC532/graphite cell comprising PEV-GPE. Flash point measurements and differential scanning calorimetry (DSC) confirmed significantly improved safety performance of PEV compared to the state-of-the-art electrolyte. PEV-GPE is a promising alternative to state-of-the-art electrolyte as it shows extended cycle life and enhanced thermal stability in NMC532/graphite lithium ion cells.
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000851197 7001_ $$0P:(DE-HGF)0$$aOnishi, Hitoshi$$b1
000851197 7001_ $$0P:(DE-Juel1)168328$$avon Aspern, Natascha$$b2$$ufzj
000851197 7001_ $$0P:(DE-HGF)0$$aRodehorst, Uta$$b3
000851197 7001_ $$0P:(DE-HGF)0$$aRudolf, Katharina$$b4
000851197 7001_ $$00000-0002-6856-9039$$aBillmann, Bastian$$b5
000851197 7001_ $$0P:(DE-HGF)0$$aWagner, Ralf$$b6
000851197 7001_ $$0P:(DE-Juel1)166130$$aWinter, Martin$$b7$$eCorresponding author$$ufzj
000851197 7001_ $$0P:(DE-Juel1)171204$$aCekic-Laskovic, Isidora$$b8$$eCorresponding author
000851197 773__ $$0PERI:(DE-600)1491915-1$$a10.1016/j.jpowsour.2018.07.039$$gVol. 397, p. 343 - 351$$p343 - 351$$tJournal of power sources$$v397$$x0378-7753$$y2018
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