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001     851197
005     20240712113113.0
024 7 _ |a 10.1016/j.jpowsour.2018.07.039
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024 7 _ |a 1873-2755
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100 1 _ |a Jia, Hao
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245 _ _ |a A propylene carbonate based gel polymer electrolyte for extended cycle life and improved safety performance of lithium ion batteries
260 _ _ |a New York, NY [u.a.]
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520 _ _ |a A poly(vinylidene difluoride-co-hexafluoropropylene) (PVdF-HFP)-based gel polymer electrolyte (GPE) containing propylene carbonate (PC)-based liquid electrolyte was developed to enhance the safety performance of LiNi0.5Mn0.3Co0.2O2/graphite (NMC532/graphite) lithium ion batteries. The PC-based liquid electrolyte (PEV-LE) consists of 1 mol L−1 LiPF6 as lithium salt, PC as the main solvent and ethylene sulfite (ES, 2% by weight) as well as vinylene carbonate (VC, 2% by weight) as solid electrolyte interphase (SEI) forming additives. Electrochemical impedance spectroscopy (EIS) and X-ray photoelectron spectroscopy (XPS) revealed that the combination of ES and VC additives facilitates the formation of effective interphases at the respective electrolyte/electrode interfaces, thus contributing to a remarkable cycle life of NMC532/graphite cell comprising PEV-GPE. Flash point measurements and differential scanning calorimetry (DSC) confirmed significantly improved safety performance of PEV compared to the state-of-the-art electrolyte. PEV-GPE is a promising alternative to state-of-the-art electrolyte as it shows extended cycle life and enhanced thermal stability in NMC532/graphite lithium ion cells.
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700 1 _ |a Onishi, Hitoshi
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700 1 _ |a von Aspern, Natascha
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700 1 _ |a Rodehorst, Uta
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700 1 _ |a Rudolf, Katharina
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700 1 _ |a Billmann, Bastian
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700 1 _ |a Wagner, Ralf
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700 1 _ |a Winter, Martin
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700 1 _ |a Cekic-Laskovic, Isidora
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773 _ _ |a 10.1016/j.jpowsour.2018.07.039
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