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@ARTICLE{Imholt:851198,
      author       = {Imholt, Laura and Dong, Dengpan and Bedrov, Dmitry and
                      Cekic-Laskovic, Isidora and Winter, Martin and Brunklaus,
                      Gunther},
      title        = {{S}upramolecular {S}elf-{A}ssembly of {M}ethylated
                      {R}otaxanes for {S}olid {P}olymer {E}lectrolyte
                      {A}pplication},
      journal      = {ACS Macro Letters},
      volume       = {7},
      number       = {7},
      issn         = {2161-1653},
      address      = {Washington, DC},
      publisher    = {ACS},
      reportid     = {FZJ-2018-04898},
      pages        = {881 - 885},
      year         = {2018},
      abstract     = {Li+-conducting solid polymer electrolytes (SPEs) obtained
                      from supramolecular self-assembly of trimethylated
                      cyclodextrin (TMCD), poly(ethylene oxide) (PEO), and lithium
                      salt are investigated for application in lithium-metal
                      batteries (LMBs) and lithium-ion batteries (LIBs). The
                      considered electrolytes comprise nanochannels for fast
                      lithium-ion transport formed by CD threaded on PEO chains.
                      It is demonstrated that tailored modification of CD
                      beneficially influences the structure and transport
                      properties of solid polymer electrolytes, thereby enabling
                      their application in LMBs. Molecular dynamics (MD)
                      simulation and experimental data reveal that modification of
                      CDs shifts the steady state between lithium ions inside and
                      outside the channels, in this way improving the achievable
                      ionic conductivity. Notably, the designed SPEs facilitated
                      galvanostatic cycling in LMBs at fast charging and
                      discharging rates for more than 200 cycles and high
                      Coulombic efficiency.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000439398500021},
      doi          = {10.1021/acsmacrolett.8b00406},
      url          = {https://juser.fz-juelich.de/record/851198},
}