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@ARTICLE{Holtstiege:851245,
author = {Holtstiege, Florian and Bärmann, Peer and Nölle, Roman
and Winter, Martin and Placke, Tobias},
title = {{P}re-{L}ithiation {S}trategies for {R}echargeable {E}nergy
{S}torage {T}echnologies: {C}oncepts, {P}romises and
{C}hallenges},
journal = {C $\–$ journal of carbon research},
volume = {4},
number = {1},
issn = {2313-0105},
address = {Basel},
publisher = {MDPI},
reportid = {FZJ-2018-04940},
pages = {4 -},
year = {2018},
abstract = {Abstract: In order to meet the sophisticated demands for
large-scale applications such as electro-mobility, next
generation energy storage technologies require advanced
electrode active materials with enhanced gravimetric and
volumetric capacities to achieve increased gravimetric
energy and volumetric energy densities. However, most of
these materials suffer from high 1st cycle active lithium
losses, e.g., caused by solid electrolyte interphase (SEI)
formation, which in turn hinder their broad commercial use
so far. In general, the loss of active lithium permanently
decreases the available energy by the consumption of lithium
from the positive electrode material. Pre-lithiation is
considered as a highly appealing technique to compensate for
active lithium losses and, therefore, to increase the
practical energy density. Various pre-lithiation techniques
have been evaluated so far, including electrochemical and
chemical pre-lithiation, pre-lithiation with the help of
additives or the pre-lithiation by direct contact to lithium
metal. In this review article, we will give a comprehensive
overview about the various concepts for pre lithiation and
controversially discuss their advantages and challenges.
Furthermore, we will critically discuss possible effects on
the cell performance and stability and assess the techniques
with regard to their possible commercial exploration.},
cin = {IEK-12},
ddc = {570},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000435206300004},
doi = {10.3390/batteries4010004},
url = {https://juser.fz-juelich.de/record/851245},
}