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000851480 1001_ $$00000-0002-5662-9866$$aPapagiannopoulos, Aristeidis$$b0$$eCorresponding author
000851480 245__ $$aAssociation and Internal Morphology of Self-Assembled HPPhOx/BSA Hybrid Nanoparticles in Aqueous Solutions
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000851480 520__ $$aWe investigate the formation of hybrid polyelectrolyte/protein nanoparticles by associations between aggregates of partially hydrolyzed poly(2-phenyl-2-oxazoline) (HPPhOx) and bovine serum albumin (BSA) in aqueous solutions. Light scattering experiments show that at conditions of low salt, BSA creates interaggregate bridges and increases the size of the HPPhOx nanoparticles. At high salt contents, breaking of aggregates leads to well-defined nanoparticles. The interior of the formed nanoparticles is probed by small-angle neutron scattering. At low salt, diffuse arrangements are observed, whereas at high salt concentration, scattering is dominated by well-defined hydrophobic domains enhanced by the incorporation of BSA. This system shows that the combination of hydrophobic and electrostatic interactions in random-amphiphilic-polyelectrolyte/protein complexes can be used to determine the properties of self-assembled hybrid multifunctional nanoparticles.
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000851480 7001_ $$0P:(DE-HGF)0$$aVlassi, Eleni$$b1
000851480 7001_ $$0P:(DE-HGF)0$$aPispas, Stergios$$b2
000851480 7001_ $$0P:(DE-Juel1)171614$$aHouston, Judith$$b3
000851480 773__ $$0PERI:(DE-600)2006039-7$$a10.1021/acs.jpcb.8b04364$$gVol. 122, no. 29, p. 7426 - 7435$$n29$$p7426 - 7435$$tThe @journal of physical chemistry <Washington, DC> / B$$v122$$x1520-5207$$y2018
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