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@ARTICLE{Giesen:851687,
author = {Giesen, Margret and Jugovac, Matteo and Zamborlini,
Giovanni and Feyer, Vitaliy and Gunkel, Felix and Müller,
David},
title = {{P}rincipal component analysis: {R}eveal camouflaged
information in x-ray absorption spectroscopy photoemission
electron microscopy of complex thin oxide films},
journal = {Thin solid films},
volume = {665},
issn = {0040-6090},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2018-05229},
pages = {75-84},
year = {2018},
abstract = {Principal component analysis (PCA) has become a standard
tool in spectromicroscopy and hyperspectral imaging to
handle large spectral data sets and to decompose raw data
into relevant and residual information. In particular in
studies of complex compounds, PCA can be used to disentangle
chemical information and thereby deepen the understanding of
chemical and physical material properties. Surprisingly, in
photoemission electron spectromicroscopy (PEEM), PCA is
rarely used. This paper serves to demonstrate how powerful
PCA can be to detect hidden chemical information in PEEM
data. We demonstrate the capability of PCA in PEEM
spectromicroscopy for the case of a thin film of a complex
quaternary oxide, Pr0.5Ba0.5CoO3-δ (PBCO) which is a main
contender catalyst material for electrocatalytic water
splitting. Upon annealing in air, PBCO decomposes into
different phases at the surface. Two of them become obvious
from the raw PEEM images, but one is revealed only after
PCA.},
cin = {PGI-6 / PGI-7},
ddc = {070},
cid = {I:(DE-Juel1)PGI-6-20110106 / I:(DE-Juel1)PGI-7-20110106},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113)},
pid = {G:(DE-HGF)POF3-113},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000447427400011},
doi = {10.1016/j.tsf.2018.09.010},
url = {https://juser.fz-juelich.de/record/851687},
}