000852442 001__ 852442 000852442 005__ 20240708134001.0 000852442 037__ $$aFZJ-2018-05388 000852442 1001_ $$0P:(DE-Juel1)144040$$aBrandt, Felix$$b0$$eCorresponding author$$ufzj 000852442 1112_ $$aGoldschmidt$$cBoston$$d2018-08-12 - 2018-08-17$$wUSA 000852442 245__ $$aRa Uptake by the Sr-Rich Solid Solution of (Sr, Ba)SO4 000852442 260__ $$c2018 000852442 3367_ $$033$$2EndNote$$aConference Paper 000852442 3367_ $$2DataCite$$aOther 000852442 3367_ $$2BibTeX$$aINPROCEEDINGS 000852442 3367_ $$2DRIVER$$aconferenceObject 000852442 3367_ $$2ORCID$$aLECTURE_SPEECH 000852442 3367_ $$0PUB:(DE-HGF)6$$2PUB:(DE-HGF)$$aConference Presentation$$bconf$$mconf$$s1537347937_29575$$xOther 000852442 520__ $$aSolid solution formation is an important mechanism of radionuclide uptake by mineral phases which is favored in natural systems due to a lowered configurational entropy. Recent studies have shown that the formationof a (Ba,Ra)SO4 solid solution significantly reduces the solubility of 226Ra in aqueous systems. This result is very relevant for the direct disposal of spent nuclear fuel in a deep geological formation, where 226Ra would dominate the dose after 100,000 years [1]. In natural systems SrSO4 often occurs along with BaSO4 implying that Ra-uptake should be assessed within the system of (Sr,Ba,Ra)SO4 + H2O. A recent thermodynamic modelling study [2] predicted a significant uptake of Ra into the ternary (Sr,Ba,Ra)SO4 solid-solution. Here we present results of long-term batch-recristallisation experiments on Ra-uptake in a Sr-rich part of the ternary system. A mechanical mixture of celestite with a small amount of barite and a (Sr,Ba)SO4 solid solution of equivalent comoposition were put into a contact with 226Ra,aq. We observed a significant uptake of 226Ra in both cases proceeding via the formation of the minor ternary Sr-, Ba- and Ra-rich phase within the major Sr-rich phase. In longer experiments the ternary phase disappeared leading to the formation of a mixture of Sr- and Ba-rich phases, within which Ra could not be detected by scanning transmission electron microscopy-energy-dispersive X-ray spetroscopy (STEM-EDX). The final 226Ra concentrations in both experiments were similar and close to predicted levels. The formation of the intermediate phase is interpreted based on structural and kinetic considerations. [1] Norrby, S. et al. (1997). “SKI SITE-94 Saekerhetsanalys foer Djupfoervar iett Kristallint berg”.Stockholm, Sweden. [2] Vinograd et al. (2018). Applied Geochemistry, in press. 000852442 536__ $$0G:(DE-HGF)POF3-161$$a161 - Nuclear Waste Management (POF3-161)$$cPOF3-161$$fPOF III$$x0 000852442 7001_ $$0P:(DE-Juel1)130364$$aKlinkenberg, Martina$$b1$$ufzj 000852442 7001_ $$0P:(DE-Juel1)169154$$aPoonoosamy, Jenna$$b2$$ufzj 000852442 7001_ $$0P:(DE-Juel1)130525$$aBarthel, Juri$$b3$$ufzj 000852442 7001_ $$0P:(DE-Juel1)157607$$aWeber, Juliane$$b4 000852442 7001_ $$0P:(DE-Juel1)130324$$aBosbach, Dirk$$b5$$ufzj 000852442 909CO $$ooai:juser.fz-juelich.de:852442$$pVDB 000852442 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)144040$$aForschungszentrum Jülich$$b0$$kFZJ 000852442 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130364$$aForschungszentrum Jülich$$b1$$kFZJ 000852442 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)169154$$aForschungszentrum Jülich$$b2$$kFZJ 000852442 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130525$$aForschungszentrum Jülich$$b3$$kFZJ 000852442 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130324$$aForschungszentrum Jülich$$b5$$kFZJ 000852442 9131_ $$0G:(DE-HGF)POF3-161$$1G:(DE-HGF)POF3-160$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lNukleare Entsorgung und Sicherheit sowie Strahlenforschung$$vNuclear Waste Management$$x0 000852442 9141_ $$y2018 000852442 9201_ $$0I:(DE-Juel1)IEK-6-20101013$$kIEK-6$$lNukleare Entsorgung und Reaktorsicherheit$$x0 000852442 9201_ $$0I:(DE-Juel1)ER-C-2-20170209$$kER-C-2$$lMaterialwissenschaft u. Werkstofftechnik$$x1 000852442 980__ $$aconf 000852442 980__ $$aVDB 000852442 980__ $$aI:(DE-Juel1)IEK-6-20101013 000852442 980__ $$aI:(DE-Juel1)ER-C-2-20170209 000852442 980__ $$aUNRESTRICTED 000852442 981__ $$aI:(DE-Juel1)IFN-2-20101013