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@ARTICLE{Anghel:852482,
author = {Anghel, Lilia and Radulescu, Aurel and Erhan, Raul Victor},
title = {{S}tructural aspects of human lactoferrin in the
iron-binding process studied by molecular dynamics and
small-angle neutron scattering},
journal = {The European physical journal / E},
volume = {41},
number = {9},
issn = {1292-895X},
address = {Berlin},
publisher = {Springer},
reportid = {FZJ-2018-05413},
pages = {109},
year = {2018},
abstract = {Lactoferrin is a non-heme protein known for its ability to
bind tightly Fe(III) ions in various physiological
environments. Due to this feature lactoferrin plays an
important role in the processes of iron regulation at the
cellular level preventing the body from damages produced by
high levels of free iron ions. The X-ray crystal structure
of human lactoferrin shows that the iron-binding process
leads to conformational changes within the protein
structure. The present study was addressed to conformation
stability of human lactoferrin in solution. Using molecular
dynamics simulations, it was shown that Arg121 is the key
amino acid in the stabilization of the Fe(III) ion in the
N-lobe of human lactoferrin. The small-angle neutron
scattering method allowed us to detect the structural
differences between the open and closed conformation of
human lactoferrin in solution. Our results indicate that the
radius of gyration of apolactoferrin appears to be smaller
than that of the hololactoferrin, Rg=24.16(±0.707) Å and
Rg=26.20(±1.191) Å, respectively. The low-resolution
three-dimensional models computed for both forms of human
lactoferrin in solution also show visible differences, both
having a more compact conformation compared to the
high-resolution structure.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
Neutron Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)KWS2-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:30229350},
UT = {WOS:000444878400002},
doi = {10.1140/epje/i2018-11720-x},
url = {https://juser.fz-juelich.de/record/852482},
}