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@ARTICLE{Jehnichen:856654,
      author       = {Jehnichen, Philipp and Wedlich, Klaus and Korte, Carsten},
      title        = {{D}egradation of {H}igh {V}oltage {C}athodes for {A}dvanced
                      {L}ithium {I}on {B}atteries - {D}ifferential {C}apacity
                      {S}tudy on {D}ifferently {B}alanced {C}ells},
      journal      = {Science and technology of advanced materials},
      volume       = {20},
      number       = {1},
      issn         = {1468-6996},
      address      = {Abingdon},
      publisher    = {Taylor $\&$ Francis},
      reportid     = {FZJ-2018-06019},
      pages        = {1-9},
      year         = {2019},
      abstract     = {The degradation of LiNi0.5Mn1.5O4 (LNMO) cathodes were
                      investigated using different cell designs (half cells, full
                      cells cathode-limited, anode-limited and cathode-limited
                      with pre-charge). Half cells based on Li/LNMO show
                      long-cycle stability due to the unlimited source of
                      electrochemically available lithium. Full-cell
                      configurations with Li4Ti5O12/LNMO are limited in their
                      cycling performance and durability. Differential capacity
                      studies during continuous cycling reveal a systematic
                      intensity change of the NiII/III and NiIII/IV redox peaks as
                      a function of the amount of electrochemically available
                      lithium. As a mechanism, it could be clearly stated that the
                      consumption of electrochemically available lithium
                      determines the cycle stability. The decomposition of the
                      active material itself (e.g. loss of Ni and Mn) is not
                      crucial for the capacity loss. Thus, full cells with a
                      pre-charged anode have the best cycling performance because
                      of its high lithium content.},
      cin          = {IEK-3},
      ddc          = {690},
      cid          = {I:(DE-Juel1)IEK-3-20101013},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000463826000001},
      doi          = {10.1080/14686996.2018.1550625},
      url          = {https://juser.fz-juelich.de/record/856654},
}