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@ARTICLE{Yalcinkaya:856730,
author = {Yalcinkaya, Hacer and Feoktystov, Artem and Gradzielski,
Michael},
title = {{F}ormation of {W}ell-{D}efined {V}esicles by {S}tyrene
{A}ddition to a {N}onionic {S}urfactant and {T}heir
{P}olymerization {L}eading to {V}iscous {H}ybrid {S}ystems},
journal = {Langmuir},
volume = {34},
number = {31},
issn = {1520-5827},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {FZJ-2018-06081},
pages = {9184 - 9194},
year = {2018},
abstract = {Self-assembled structures in aqueous solutions can be fixed
by polymerization after adding hydrophobic monomers and can
thereby be used as templates which allows to substantially
alter the properties of these systems. In this work, we
started from a self-assembled micellar system consisting of
the nonionic surfactants tetradecyldimethylamine oxid
(TDMAO) and Pluronic L35 to which styrene was added as a
polymerizable monomer. Interestingly, it was observed that
styrene induces a transition from micelles to well-defined
vesicles in a similar manner as a typical cosurfactant. The
structural transition of the aggregates upon styrene
addition as well as the structures formed after initiating a
polymerization reaction were investigated by means of
turbidity, dynamic and static light scattering, (DLS, SLS),
small angle neutron scattering (SANS), and rheology
measurements. Especially the scattering results confirmed
the interesting effect of styrene on the mesoscopic
structure and showed a structural evolution from rod-like
micelles for low styrene concentrations to vesicles at
intermediate styrene amounts, and then finally the formation
of microemulsion droplets for high styrene content. Their
polymerization of the vesicles again leads to a shape change
to wormlike, polymerized aggregates, whose presence then
results in rather viscous systems. In contrast, the
microemulsions with higher styrene content then are
templated and retain their size after polymerization,
thereby leading to nanolatices.},
cin = {JCNS-FRM-II / JCNS-2},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6G15 - FRM II / MLZ (POF3-6G15)},
pid = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
experiment = {EXP:(DE-MLZ)KWS1-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:30010346},
UT = {WOS:000441477300009},
doi = {10.1021/acs.langmuir.8b01377},
url = {https://juser.fz-juelich.de/record/856730},
}