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@ARTICLE{Tan:857700,
      author       = {Tan, Zhaofeng and Lu, Keding and Dong, Huabin and Hu, Min
                      and Li, Xin and Liu, Yuhan and Lu, Sihua and Shao, Min and
                      Su, Rong and Wang, Haichao and Wu, Yusheng and Wahner,
                      Andreas and Zhang, Yuanhang},
      title        = {{E}xplicit diagnosis of the local ozone production rate and
                      the ozone-{NO}x-{VOC} sensitivities},
      journal      = {Science bulletin},
      volume       = {63},
      number       = {16},
      issn         = {2095-9273},
      address      = {[S.l.]},
      publisher    = {Science China Press},
      reportid     = {FZJ-2018-06672},
      pages        = {1067 - 1076},
      year         = {2018},
      abstract     = {In the troposphere, ozone is a harmful gas compound to both
                      human health and vegetation. Ozone is produced from the
                      reaction of NOx (NO + NO2) and VOCs (volatile organic
                      compounds) with light. Due to the highly nonlinear
                      relationships between ozone and its precursors, proper ozone
                      mitigation relies on the knowledge of chemical mechanisms.
                      In this study, an observation-based method is used to
                      simulate ozone formation and elucidate its controlling
                      factors for a rural site on the North China Plain. The
                      instantaneous ozone production rate is calculated utilizing
                      a box model using the dataset obtained from the Wangdu
                      campaign. First, the model was operated in a time-dependent
                      mode to calculate the ozone production rate at each time
                      stamp. The calculated ozone formation rate showed a diurnal
                      average maximum value of 17 ppbv/h (1-h diurnal averaged).
                      The contribution of individual peroxy radicals to ozone
                      production was analyzed. In addition, the functional
                      dependence of calculated P(O3) reveals that ozone production
                      was in a NOx-limited regime during the campaign.
                      Furthermore, the missing peroxy radical source will further
                      extend NOx-limited conditions to earlier in the day, making
                      NOx limitation dominate more of a day than the current
                      chemical model predicts. Finally, a multiple scenarios mode,
                      also known as EKMA (empirical kinetic modeling approach),
                      was used to simulate the response of P(O3) to the imaginary
                      change in precursor concentrations. We found that ozone
                      production was in the NOx-limited region. However, the use
                      of NO2 measured by the molybdenum converter and/or the
                      absence of a peroxy radical source in the current chemical
                      model could over-emphasize the VOC-limited effect on ozone
                      production.},
      cin          = {IEK-8},
      ddc          = {500},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000442738700014},
      doi          = {10.1016/j.scib.2018.07.001},
      url          = {https://juser.fz-juelich.de/record/857700},
}