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@ARTICLE{GomezMartin:857800,
author = {Gomez-Martin, Aurora and Martinez-Fernandez, Julian and
Ruttert, Mirco and Heckmann, Andreas and Winter, Martin and
Placke, Tobias and Ramirez-Rico, Joaquin},
title = {{I}ron-{C}atalyzed {G}raphitic {C}arbon {M}aterials from
{B}iomass {R}esources as {A}nodes for {L}ithium-{I}on
{B}atteries},
journal = {ChemSusChem},
volume = {11},
number = {16},
issn = {1864-5631},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2018-06767},
pages = {2776 - 2787},
year = {2018},
abstract = {Graphitized carbon materials from biomass resources were
successfully synthesized with an iron catalyst, and their
electrochemical performance as anode materials for
lithium‐ion batteries (LIBs) was investigated. Peak
pyrolysis temperatures between 850 and 2000 °C were
covered to study the effect of crystallinity and
microstructural parameters on the anodic behavior, with a
focus on the first‐cycle Coulombic efficiency, reversible
specific capacity, and rate performance. In terms of
capacity, results at the highest temperatures are comparable
to those of commercially used synthetic graphite derived
from a petroleum coke precursor at higher temperatures, and
up to twice as much as that of uncatalyzed biomass‐derived
carbons. The opportunity to graphitize low‐cost biomass
resources at moderate temperatures through this one‐step
environmentally friendly process, and the positive effects
on the specific capacity, make it interesting to develop
more sustainable graphite‐based anodes for LIBs.},
cin = {IEK-12},
ddc = {540},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:29870144},
UT = {WOS:000442491300017},
doi = {10.1002/cssc.201800831},
url = {https://juser.fz-juelich.de/record/857800},
}