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@ARTICLE{Jia:857829,
      author       = {Jia, Hao and Onishi, Hitoshi and Wagner, Ralf and Winter,
                      Martin and Cekic-Laskovic, Isidora},
      title        = {{A}n {I}ntrinsically {S}afe {G}el {P}olymer {E}lectrolyte
                      {C}omprising {F}lame {R}etarding {P}olymer {M}atrix for
                      {L}ithium {I}on {B}attery {A}pplication},
      journal      = {ACS applied materials $\&$ interfaces},
      volume       = {10},
      number       = {49},
      issn         = {1944-8252},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2018-06796},
      pages        = {42348-42355},
      year         = {2018},
      abstract     = {State-of-the-art (SOTA) liquid electrolyte/polyolefin
                      separator setups used in lithium ion batteries suffer from
                      the hazard of leakage and high flammability. To address
                      these issues, phosphonate, a flame retarding moiety, is
                      chemically bonded to a polymer matrix to fabricate a
                      non-flammable gel polymer electrolyte (GPE). The obtained
                      phosphonate-based polymer matrix as well as its
                      corresponding GPE (gelled with flammable SOTA non-aqueous
                      liquid electrolyte) show remarkable flame resistivity.
                      Unlike poly(vinylidene fluoride-co-hexafluoropropylene)
                      (PVdF-HFP)-based GPEs, the phosphonate-based GPE does not
                      react with lithiated graphite at high temperatures. Both
                      features indicate that the phosphonate-based GPE is superior
                      to SOTA GPEs in the aspect of safety performance. As the
                      flame retarding moiety is chemically bonding to the polymer,
                      the parasitic reactions between the flame retarding moiety
                      and the electrodes are avoided. Consequently, lithium ion
                      battery (LIB) cells comprising phosphonate-based GPE show
                      good capacity retention comparable to cells comprising SOTA
                      GPEs. Compared with SOTA GPEs, phosphonate-based polymer
                      based GPEs show improved intrinsic safety performance and
                      comparable cycle life. Therefore, phosphonate-based polymers
                      exhibit high potential to be used as a new class of polymer
                      matrix for GPE used in LIBs.},
      cin          = {IEK-12},
      ddc          = {600},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:30403125},
      UT           = {WOS:000453488900055},
      doi          = {10.1021/acsami.8b15505},
      url          = {https://juser.fz-juelich.de/record/857829},
}