000857840 001__ 857840
000857840 005__ 20240709082127.0
000857840 0247_ $$2doi$$a10.1002/aenm.201802404
000857840 0247_ $$2ISSN$$a1614-6832
000857840 0247_ $$2ISSN$$a1614-6840
000857840 0247_ $$2WOS$$aWOS:000453273200003
000857840 0247_ $$2altmetric$$aaltmetric:50587458
000857840 037__ $$aFZJ-2018-06807
000857840 041__ $$aEnglish
000857840 082__ $$a050
000857840 1001_ $$0P:(DE-HGF)0$$aRodenas, Tania$$b0$$eCorresponding author
000857840 245__ $$a2D Metal Organic Framework-Graphitic Carbon Nanocomposites as Precursors for High-Performance O 2 -Evolution Electrocatalysts
000857840 260__ $$aWeinheim$$bWiley-VCH$$c2018
000857840 3367_ $$2DRIVER$$aarticle
000857840 3367_ $$2DataCite$$aOutput Types/Journal article
000857840 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1544879664_22109
000857840 3367_ $$2BibTeX$$aARTICLE
000857840 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000857840 3367_ $$00$$2EndNote$$aJournal Article
000857840 520__ $$aThe development of effective and precious‐metal‐free electrocatalysts for the oxygen evolution reaction (OER) represents a major bottleneck to unlock a renewable energy scenario based on water splitting technologies. Materials uniting the electrical conductivity of conjugated graphitic nanomaterials with the chemical regularity of metal‐organic‐framework (MOF) crystals are promising precursors for such electrocatalysts. Nanoscale integration of these two materials is challenging. A new synthesis route is developed that integrates 2D MOF nanocrystals and graphitic carbon nanolamellae into layered composites. The graphitic carrier contributes excellent charge–transport properties, and the 2D macromolecular MOF precursor provides a suitable shuttle for introducing highly dispersed metal species. Furthermore their direct chemical environment can be controlled via selection of organic linker. Thermal decomposition of 2D cobalt tetrafluoro benzene‐dicarboxylate MOF nanocrystals within such composites enables the stabilization of cobalt oxyhydroxyfluoride nanoparticles on the graphitic carrier, which display an extraordinary activity for the OER in alkaline media, with low onset overpotential (310 mVRHE) and current densities >104 mA cm−2 μmolCo−1 at an operating overpotential of 450 mV, alongside excellent operational stability. The wide compositional array of MOFs makes this synthesis approach versatile toward advanced (electro)catalysts and other functional materials for applications from sensing to energy storage and conversion.
000857840 536__ $$0G:(DE-HGF)POF3-131$$a131 - Electrochemical Storage (POF3-131)$$cPOF3-131$$fPOF III$$x0
000857840 588__ $$aDataset connected to CrossRef
000857840 7001_ $$0P:(DE-HGF)0$$aBeeg, Sebastian$$b1
000857840 7001_ $$0P:(DE-HGF)0$$aSpanos, Ioannis$$b2
000857840 7001_ $$0P:(DE-HGF)0$$aNeugebauer, Sebastian$$b3
000857840 7001_ $$0P:(DE-HGF)0$$aGirgsdies, Frank$$b4
000857840 7001_ $$0P:(DE-HGF)0$$aAlgara-Siller, Gerardo$$b5
000857840 7001_ $$0P:(DE-Juel1)168465$$aSchleker, Peter Philipp Maria$$b6
000857840 7001_ $$0P:(DE-Juel1)156296$$aJakes, Peter$$b7
000857840 7001_ $$0P:(DE-HGF)0$$aPfänder, Norbert$$b8
000857840 7001_ $$0P:(DE-HGF)0$$aWillinger, Marc$$b9
000857840 7001_ $$0P:(DE-HGF)0$$aGreiner, Mark$$b10
000857840 7001_ $$0P:(DE-HGF)0$$aPrieto, Gonzalo$$b11
000857840 7001_ $$0P:(DE-HGF)0$$aSchlögl, Robert$$b12
000857840 7001_ $$00000-0003-3594-6392$$aHeumann, Saskia$$b13
000857840 773__ $$0PERI:(DE-600)2594556-7$$a10.1002/aenm.201802404$$gp. 1802404 -$$n35$$p1802404 -$$tAdvanced energy materials$$v8$$x1614-6832$$y2018
000857840 909CO $$ooai:juser.fz-juelich.de:857840$$pVDB
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b0
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b1
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b2
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b3
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aExternal Institute$$b4$$kExtern
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b4
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b5
000857840 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)168465$$aForschungszentrum Jülich$$b6$$kFZJ
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)168465$$aMPI-CEC Mülheim $$b6
000857840 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)156296$$aForschungszentrum Jülich$$b7$$kFZJ
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b8
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b9
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b10
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI-CEC Mülheim $$b11
000857840 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aMPI Mülheim $$b12
000857840 9101_ $$0I:(DE-HGF)0$$60000-0003-3594-6392$$aMPI-CEC Mülheim $$b13
000857840 9131_ $$0G:(DE-HGF)POF3-131$$1G:(DE-HGF)POF3-130$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lSpeicher und vernetzte Infrastrukturen$$vElectrochemical Storage$$x0
000857840 9141_ $$y2018
000857840 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000857840 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000857840 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bADV ENERGY MATER : 2017
000857840 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search
000857840 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC
000857840 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List
000857840 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000857840 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000857840 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000857840 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology
000857840 915__ $$0StatID:(DE-HGF)9920$$2StatID$$aIF >= 20$$bADV ENERGY MATER : 2017
000857840 920__ $$lyes
000857840 9201_ $$0I:(DE-Juel1)IEK-9-20110218$$kIEK-9$$lGrundlagen der Elektrochemie$$x0
000857840 980__ $$ajournal
000857840 980__ $$aVDB
000857840 980__ $$aI:(DE-Juel1)IEK-9-20110218
000857840 980__ $$aUNRESTRICTED
000857840 981__ $$aI:(DE-Juel1)IET-1-20110218