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@ARTICLE{Rodenas:857840,
      author       = {Rodenas, Tania and Beeg, Sebastian and Spanos, Ioannis and
                      Neugebauer, Sebastian and Girgsdies, Frank and
                      Algara-Siller, Gerardo and Schleker, Peter Philipp Maria and
                      Jakes, Peter and Pfänder, Norbert and Willinger, Marc and
                      Greiner, Mark and Prieto, Gonzalo and Schlögl, Robert and
                      Heumann, Saskia},
      title        = {2{D} {M}etal {O}rganic {F}ramework-{G}raphitic {C}arbon
                      {N}anocomposites as {P}recursors for {H}igh-{P}erformance
                      {O} 2 -{E}volution {E}lectrocatalysts},
      journal      = {Advanced energy materials},
      volume       = {8},
      number       = {35},
      issn         = {1614-6832},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2018-06807},
      pages        = {1802404 -},
      year         = {2018},
      abstract     = {The development of effective and precious‐metal‐free
                      electrocatalysts for the oxygen evolution reaction (OER)
                      represents a major bottleneck to unlock a renewable energy
                      scenario based on water splitting technologies. Materials
                      uniting the electrical conductivity of conjugated graphitic
                      nanomaterials with the chemical regularity of
                      metal‐organic‐framework (MOF) crystals are promising
                      precursors for such electrocatalysts. Nanoscale integration
                      of these two materials is challenging. A new synthesis route
                      is developed that integrates 2D MOF nanocrystals and
                      graphitic carbon nanolamellae into layered composites. The
                      graphitic carrier contributes excellent charge–transport
                      properties, and the 2D macromolecular MOF precursor provides
                      a suitable shuttle for introducing highly dispersed metal
                      species. Furthermore their direct chemical environment can
                      be controlled via selection of organic linker. Thermal
                      decomposition of 2D cobalt tetrafluoro
                      benzene‐dicarboxylate MOF nanocrystals within such
                      composites enables the stabilization of cobalt
                      oxyhydroxyfluoride nanoparticles on the graphitic carrier,
                      which display an extraordinary activity for the OER in
                      alkaline media, with low onset overpotential (310 mVRHE) and
                      current densities >104 mA cm−2 μmolCo−1 at an operating
                      overpotential of 450 mV, alongside excellent operational
                      stability. The wide compositional array of MOFs makes this
                      synthesis approach versatile toward advanced
                      (electro)catalysts and other functional materials for
                      applications from sensing to energy storage and conversion.},
      cin          = {IEK-9},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000453273200003},
      doi          = {10.1002/aenm.201802404},
      url          = {https://juser.fz-juelich.de/record/857840},
}