TY - JOUR
AU - Panwalkar, Vineet
AU - Neudecker, Philipp
AU - Willbold, Dieter
AU - Dingley, Andrew J.
TI - Multiple WW domains of Nedd4-1 undergo conformational exchange that is quenched upon peptide binding
JO - FEBS letters
VL - 591
IS - 11
SN - 0014-5793
CY - Chichester
PB - Wiley
M1 - FZJ-2018-06835
SP - 1573 - 1583
PY - 2017
AB - The third WW domain (WW3*) of the ubiquitin ligase human neuronal precursor cell expressed developmentally downregulated gene 4-1 (hNedd4-1) was reported to bind its PY motif peptide by a coupled folding-binding equilibrium. However, it is unknown whether these thermodynamic properties are retained in the context of neighboring hNedd4-1 domains. In this report, NMR data show that the WW3* displays a fold-unfold equilibrium in the presence of neighboring WW domains, and that similar fold-unfold equilibria also likely exist for neighboring WW domains. These equilibria are quenched upon interaction with peptide. Thus, the binding mechanism of hNedd4-1 WW domains to proteins involves coupled folding and binding equilibria, and this mechanism may be a general feature that modulates peptide affinities of WW domains.
LB - PUB:(DE-HGF)16
C6 - pmid:28471472
UR - <Go to ISI:>//WOS:000403354400009
DO - DOI:10.1002/1873-3468.12664
UR - https://juser.fz-juelich.de/record/857872
ER -