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@ARTICLE{Kehne:857919,
author = {Kehne, P. and Guhl, C. and Ma, Qianli and Tietz, F. and
Alff, L. and Hausbrand, R. and Komissinskiy, P.},
title = {{S}c-substituted {N}asicon solid electrolyte for an
all-solid-state {N}ax{C}o{O}2/{N}asicon/{N}a sodium model
battery with stable electrochemical performance},
journal = {Journal of power sources},
volume = {409},
issn = {0378-7753},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2018-06873},
pages = {86 - 93},
year = {2019},
abstract = {All-solid-state sodium batteries are attractive due to the
abundance of sodium and advantageous for safe battery
operation by avoiding flammable organics and liquids and
suppressed dendrite formation. Currently, the lack of a
chemically stable sodium solid electrolyte with high ion
conductivity at room temperature is one of the challenges
for future development of sodium batteries. Herein, we
present a NaxCoO2/Nasicon/Na thin-film model sodium
solid-state battery using a Sc-substituted Nasicon solid
electrolyte with a high ionic conductivity of 4 × 10⁻³ S
cm⁻¹. The battery shows a high specific capacity of 150
mAh g⁻¹ at room-temperature and discharge rates of up to
6C. Excellent chemical stability of this solid electrolyte
at high voltages of up to 4.2 V increases the accessible
sodium (de)intercalation range and battery capacity. Direct
extraction of the interface resistances between the
electrode materials of the thin-film model cell using
electrochemical impedance spectroscopy gives a unique
opportunity of correlation the electrochemical performance
with properties of electrode materials and their
interfaces.},
cin = {IEK-1},
ddc = {620},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000452945600011},
doi = {10.1016/j.jpowsour.2018.10.089},
url = {https://juser.fz-juelich.de/record/857919},
}