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@ARTICLE{Faisal:858239,
      author       = {Faisal, Firas and Stumm, Corinna and Bertram, Manon and
                      Waidhas, Fabian and Lykhach, Yaroslava and Cherevko, Serhiy
                      and Xiang, Feifei and Ammon, Maximilian and Vorokhta,
                      Mykhailo and Šmíd, Břetislav and Skála, Tomáš and
                      Tsud, Nataliya and Neitzel, Armin and Beranová, Klára and
                      Prince, Kevin C. and Geiger, Simon and Kasian, Olga and
                      Wähler, Tobias and Schuster, Ralf and Schneider, M.
                      Alexander and Matolín, Vladimír and Mayrhofer, Karl and
                      Brummel, Olaf and Libuda, Jörg},
      title        = {{E}lectrifying model catalysts for understanding
                      electrocatalytic reactions in liquid electrolytes},
      journal      = {Nature materials},
      volume       = {17},
      number       = {7},
      issn         = {1476-4660},
      address      = {Basingstoke},
      publisher    = {Nature Publishing Group},
      reportid     = {FZJ-2018-07139},
      pages        = {592 - 598},
      year         = {2018},
      abstract     = {Electrocatalysis is at the heart of our future transition
                      to a renewable energy system. Most energy storage and
                      conversion technologies for renewables rely on
                      electrocatalytic processes and, with increasing availability
                      of cheap electrical energy from renewables, chemical
                      production will witness electrification in the near
                      future1,2,3. However, our fundamental understanding of
                      electrocatalysis lags behind the field of classical
                      heterogeneous catalysis that has been the dominating
                      chemical technology for a long time. Here, we describe a new
                      strategy to advance fundamental studies on electrocatalytic
                      materials. We propose to ‘electrify’ complex oxide-based
                      model catalysts made by surface science methods to explore
                      electrocatalytic reactions in liquid electrolytes. We
                      demonstrate the feasibility of this concept by transferring
                      an atomically defined platinum/cobalt oxide model catalyst
                      into the electrochemical environment while preserving its
                      atomic surface structure. Using this approach, we explore
                      particle size effects and identify hitherto unknown
                      metal–support interactions that stabilize oxidized
                      platinum at the nanoparticle interface. The metal–support
                      interactions open a new synergistic reaction pathway that
                      involves both metallic and oxidized platinum. Our results
                      illustrate the potential of the concept, which makes
                      available a systematic approach to build atomically defined
                      model electrodes for fundamental electrocatalytic studies.},
      cin          = {IEK-11 / JARA-HPC},
      ddc          = {610},
      cid          = {I:(DE-Juel1)IEK-11-20140314 / $I:(DE-82)080012_20140620$},
      pnm          = {134 - Electrolysis and Hydrogen (POF3-134) / Ab initio
                      study of amorphous Sb $(jara0176_20171101)$},
      pid          = {G:(DE-HGF)POF3-134 / $G:(DE-Juel1)jara0176_20171101$},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:29867166},
      UT           = {WOS:000436341400012},
      doi          = {10.1038/s41563-018-0088-3},
      url          = {https://juser.fz-juelich.de/record/858239},
}