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@ARTICLE{Stopic:858264,
      author       = {Stopic, Srecko and Dertmann, Christian and Modolo, Giuseppe
                      and Kegler, Philip and Neumeier, Stefan and Kremer, Dario
                      and Wotruba, Hermann and Etzold, Simon and Telle, Rainer and
                      Rosani, Diego and Knops, Pol and Friedrich, Bernd},
      title        = {{S}ynthesis of {M}agnesium {C}arbonate via {C}arbonation
                      under {H}igh {P}ressure in an {A}utoclave},
      journal      = {Metals},
      volume       = {8},
      number       = {12},
      issn         = {2075-4701},
      address      = {Basel},
      publisher    = {MDPI},
      reportid     = {FZJ-2018-07159},
      pages        = {993 -},
      year         = {2018},
      abstract     = {Magnesium carbonate powders are essential in the
                      manufacture of basic refractories capable of withstanding
                      extremely high temperatures and for special types of cement
                      and powders used in the paper, rubber, and pharmaceutical
                      industries. A novel synthesis route is based on CO2
                      absorption/sequestration by minerals. This combines the
                      global challenge of climate change with materials
                      development. Carbon dioxide has the fourth highest
                      composition in earth’s atmosphere next to nitrogen, oxygen
                      and argon and plays a big role in global warming due to the
                      greenhouse effect. Because of the significant increase of
                      CO2 emissions, mineral carbonation is a promising process in
                      which carbon oxide reacts with materials with high metal
                      oxide composition to form chemically stable and insoluble
                      metal carbonate. The formed carbonate has long-term
                      stability and does not influence the earth’s atmosphere.
                      Therefore, it is a feasible and safe method to bind carbon
                      dioxide in carbonate compounds such as magnesite. The
                      subject of this work is the carbonation of an olivine
                      (Mg2SiO4) and synthetic magnesia sample (>97 $wt\%$ MgO)
                      under high pressure and temperature in an autoclave. Early
                      experiments have studied the influence of some additives
                      such as sodium bicarbonate, oxalic acid and ascorbic acid,
                      solid/liquid ratio, and particle size on the carbonation
                      efficiency. The obtained results for carbonation of olivine
                      have confirmed the formation of magnesium carbonate in the
                      presence of additives and complete carbonation of the MgO
                      sample in the absence of additives},
      cin          = {IEK-6},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-6-20101013},
      pnm          = {161 - Nuclear Waste Management (POF3-161)},
      pid          = {G:(DE-HGF)POF3-161},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000455072100017},
      doi          = {10.3390/met8120993},
      url          = {https://juser.fz-juelich.de/record/858264},
}