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@ARTICLE{Qaim:858324,
author = {Qaim, Syed M. and Scholten, Bernhard and Neumaier, Bernd},
title = {{N}ew developments in the production of theranostic pairs
of radionuclides},
journal = {Journal of radioanalytical and nuclear chemistry},
volume = {318},
number = {3},
issn = {1588-2780},
address = {Dordrecht [u.a.]},
publisher = {Springer Science + Business Media B.V},
reportid = {FZJ-2018-07212},
pages = {1493 - 1509},
year = {2018},
abstract = {A brief historical background of the development of the
theranostic approach in nuclear medicine is given and seven
theranostic pairs of radionuclides, namely 44gSc/47Sc,
64Cu/67Cu, 83Sr/89Sr, 86Y/90Y, 124I/131I, 152Tb/161Tb and
152Tb/149Tb, are considered. The first six pairs consist of
a positron and a β−-emitter whereas the seventh pair
consists of a positron and an α-particle emitter. The decay
properties of all those radionuclides are briefly mentioned
and their production methodologies are discussed. The
positron emitters 64Cu, 86Y and 124I are commonly produced
in sufficient quantities via the (p,n) reaction on the
respective highly enriched target isotope. A clinical scale
production of the positron emitter 44gSc has been achieved
via the generator route as well as via the (p,n) reaction,
but further development work is necessary. The positron
emitters 83Sr and 152Tb are under development. Among the
therapeutic radionuclides, 89Sr, 90Y and 131I are
commercially available and 161Tb can also be produced in
sufficient quantity at a nuclear reactor. Great efforts are
presently underway to produce 47Sc and 67Cu via neutron,
photon and charged particle induced reactions. The
radionuclide 149Tb is unique because it is an α-particle
emitter. The present method of production of 152Tb and 149Tb
involves the use of the spallation process in combination
with an on-line mass separator. The role of some emerging
irradiation facilities in the production of special
radionuclides is discussed.},
cin = {INM-5},
ddc = {540},
cid = {I:(DE-Juel1)INM-5-20090406},
pnm = {573 - Neuroimaging (POF3-573)},
pid = {G:(DE-HGF)POF3-573},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000451746300005},
doi = {10.1007/s10967-018-6238-x},
url = {https://juser.fz-juelich.de/record/858324},
}