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@ARTICLE{Wang:858486,
author = {Wang, Hao and Eze, Peter M. and Höfert, Simon-Patrick and
Janiak, Christoph and Hartmann, Rudolf and Okoye, Festus B.
C. and Esimone, Charles O. and Orfali, Raha S. and Dai,
Haofu and Liu, Zhen and Proksch, Peter},
title = {{S}ubstituted l -tryptophan- l -phenyllactic acid
conjugates produced by an endophytic fungus {A}spergillus
aculeatus using an {OSMAC} approach},
journal = {RSC Advances},
volume = {8},
number = {14},
issn = {2046-2069},
address = {London},
publisher = {RSC Publishing},
reportid = {FZJ-2018-07358},
pages = {7863 - 7872},
year = {2018},
abstract = {The endophytic fungus Aspergillus aculeatus isolated from
leaves of the papaya plant Carica papaya was fermented on
solid rice medium, yielding a new
L-tryptophan-L-phenyllactic acid conjugate (1) and thirteen
known compounds (11, 14–25). In addition, an OSMAC
approach was employed by adding eight different sodium or
ammonium salts to the rice medium. Addition of $3.5\%$ NaNO3
caused a significant change of the metabolite pattern of the
fungus as indicated by HPLC analysis. Subsequent isolation
yielded several new substituted L-tryptophan-L-phenyllactic
acid conjugates (1–10) in addition to three known
compounds (11–13), among which compounds 2–10, 12–13
were not detected in the rice control culture. All
structures were unambiguously elucidated by one and two
dimensional NMR spectroscopy and by mass spectrometry. The
absolute configuration of the new compounds was determined
by Marfey's reaction and X-ray single crystal diffraction.
Compounds 19–22 showed cytotoxicity against the L5178Y
mouse lymphoma cell line with IC50 values of 3.4, 1.4, 7.3
and 23.7 μM, respectively.},
cin = {ICS-6},
ddc = {540},
cid = {I:(DE-Juel1)ICS-6-20110106},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551)},
pid = {G:(DE-HGF)POF3-551},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000425647000062},
doi = {10.1039/C8RA00200B},
url = {https://juser.fz-juelich.de/record/858486},
}