TY - JOUR
AU - Grasmik, Viktoria
AU - Breisch, Marina
AU - Loza, Kateryna
AU - Heggen, Marc
AU - Köller, Manfred
AU - Sengstock, Christina
AU - Epple, Matthias
TI - Synthesis and biological characterization of alloyed silver–platinum nanoparticles: from compact core–shell nanoparticles to hollow nanoalloys
JO - RSC Advances
VL - 8
IS - 67
SN - 2046-2069
CY - London
PB - RSC Publishing
M1 - FZJ-2018-07467
SP - 38582 - 38590
PY - 2018
AB - Bimetallic nanoparticles consisting of silver and platinum were prepared by a modified seeded-growth process in water in the full composition range in steps of 10 mol%. The particles had diameters between 15–25 nm as determined by disc centrifugal sedimentation (DCS) and transmission electron microscopy (TEM). Whereas particles with high platinum content were mostly spherical with a solid silver core/platinum shell structure, mostly hollow alloyed nanoparticles were observed with increasing silver content. The internal structure and the elemental distribution within the particles were elucidated by high-resolution transmission electron microscopy (HRTEM) in combination with energy-dispersive X-ray spectroscopy (EDX). The particles were cytotoxic for human mesenchymal stem cells (hMSC) above 50 mol% silver. This was explained by dissolution experiments where silver was only released at and above 50 mol% silver. In contrast, platinum-rich particles (less than 50 mol% silver) did not release any silver ions. This indicates that the presence of platinum inhibits the oxidative dissolution of silver.
LB - PUB:(DE-HGF)16
UR - <Go to ISI:>//WOS:000451075500051
DO - DOI:10.1039/C8RA06461J
UR - https://juser.fz-juelich.de/record/858607
ER -