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@ARTICLE{Stuckart:858635,
      author       = {Stuckart, Maria and Monakhov, Kirill},
      title        = {{P}olyoxometalate encapsulation into metal–organic
                      frameworks: the way towards functional nanomaterials for
                      water splitting},
      journal      = {Journal of materials chemistry / A Materials for energy and
                      sustainability A},
      volume       = {6},
      number       = {37},
      issn         = {2050-7496},
      address      = {London},
      publisher    = {RSC72819},
      reportid     = {FZJ-2018-07494},
      pages        = {17849 - 17853},
      year         = {2018},
      abstract     = {Today, the trapping of polyoxometalates (POMs) into
                      different molecular assemblies represents a new emerging
                      field of study. Herein we show the benefits of POM
                      incorporation based on the example of a recently published
                      achievement in the area of metal–organic frameworks
                      (MOFs), where the transformation of low-cost
                      noble-metal-free Keggin-POM@MOF hybrids through pyrolysis
                      leads to small-sized bi-transition metal carbide particles
                      opening up far-reaching opportunities for water splitting.
                      The peculiarities of synthesis and reactivity of these
                      unconventional Keggin-POM@MOF compounds are described. The
                      bifunctional electrocatalytic activity of nanoparticles
                      fabricated from the hybrids is emphasised with regard to
                      reported catalytic systems of the same type. Overall, the
                      synthetic strategy reported is expected to be used for the
                      preparation of a novel type of POM@MOF hybrid where
                      polyoxoanions are not only encapsulated in the MOF cages as
                      commonly observed but also partially fenced by them, while
                      blocking the POM withdrawal. This promises diverse
                      attractive application prospects for POM@MOF hybrids in
                      heterogeneous catalysis.},
      cin          = {PGI-6 / JARA-FIT},
      ddc          = {530},
      cid          = {I:(DE-Juel1)PGI-6-20110106 / $I:(DE-82)080009_20140620$},
      pnm          = {522 - Controlling Spin-Based Phenomena (POF3-522)},
      pid          = {G:(DE-HGF)POF3-522},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000448340100001},
      doi          = {10.1039/C8TA06213G},
      url          = {https://juser.fz-juelich.de/record/858635},
}