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@INPROCEEDINGS{Park:858755,
author = {Park, Gunwoo and Ianniruberto, G.},
title = {{E}xploring {S}hear {T}hickening of {T}elechelic
{A}ssociating {P}olymers through {S}tochastic {S}imulations},
reportid = {FZJ-2018-07600},
year = {2018},
abstract = {Hydrophobically modified exthoxylated urethane (HEUR) is
one of the most popular examples of telechelic associating
polymer. In a certain range of HEUR concentration in aqueous
solution, (i) linear viscoelasticity follows a
single-Maxwellian behavior with a characteristic time
controlled by the network relaxation due to
association/dissociation kinetics. In simple shear flows,
HEUR systems often (ii) exhibit strain hardening in the
transient startup when the shear rate exceeds the reciprocal
relaxation time, and (iii) at steady state deviate from the
Cox-Merz rule, deviations including (iv) a shear-thickening
phenomenon. Recently, Park and Ianniruberto [1] suggested a
new stochastic simulation to describe the complex
rheological behavior listed in (i-iv). The results indicate
that finite extensibility effects are mostly responsible for
the strain hardening, while deviations from the Cox-Merz
rule are due to the persistence of bridge chains. However,
the detailed mechanism behind the shear thickening is still
unclear. In this study, we show additional observables by
using the same simulation method for a better understanding
of the shear-thickening phenomenon. Furthermore, we extend
the range of the parameter space explored in [1] by
examining larger (and more reasonable) values of the ratio
between the loop dissociation time and the Brownian
diffusion time of flower-like micelles. [1] G. W. Park and
G. Ianniruberto, J. Rheol. 61, 1293 (2017)},
month = {Apr},
date = {2018-04-17},
organization = {Annual European Rheology Conference
2018, Sorrento (Italy), 17 Apr 2018 -
20 Apr 2018},
subtyp = {After Call},
cin = {ICS-3},
cid = {I:(DE-Juel1)ICS-3-20110106},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551) /
SFB 985 B06 - Kontinuierliche Trennung und Aufkonzentrierung
von Mikrogelen (B06) (221475706)},
pid = {G:(DE-HGF)POF3-551 / G:(GEPRIS)221475706},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/858755},
}