% IMPORTANT: The following is UTF-8 encoded. This means that in the presence
% of non-ASCII characters, it will not work with BibTeX 0.99 or older.
% Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or
% “biber”.
@ARTICLE{Sehnem:859035,
author = {Sehnem, André Luiz and Neto, Antônio Martins Figueiredo
and Niether, Doreen and Wiegand, Simone},
title = {{D}iffusiophoresis as ruling effect: {I}nfluence of organic
salts on thermodiffusion of iron oxide nanoparticles},
journal = {Physical review / E},
volume = {98},
number = {6},
issn = {2470-0045},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2019-00005},
pages = {062615},
year = {2018},
abstract = {Colloidal particles, including ferrofluidic nanoparticles
(NP), move in a temperature gradient due to thermodiffusion.
Organic salts, which are often added to disperse the NP in
aqueous solution, also move in the temperature gradient.
This can have a strong influence on the behaviour of the NP,
which not only respond to the temperature gradient, but also
to the concentration gradient of the dispersive salt, an
effect termed diffusiophoresis. In this work we present
experimental results on thermodiffusion of iron oxide
nanoparticlesdispersed in aqueous solutions of organic
hydroxides, which illustrate $\%the$ possibility of
expressive changes in thermodiffusion of nanoparticles. the
possibility to manipulate the thermodiffusion of NP through
the addition of organic salts. Our experiments investigate
the temperature dependence of the particles' Soret
coefficient, a recurring question on thermodiffusion of
water dispersed particles. Existing theoretical approaches
are compared and we relate the Soret coefficient of the NP
with two main physical parameters ruling particle motion:
the NP's electrostatic potential and the Soret coefficient
of the dispersing ions. These parameters are also
experimentally determined. At the order of magnitude of the
NP's Soret coefficient good agreement between experiments
and theory is achieved by including the experimental data on
the Soret coefficient of the dispersing ions and therefore
the NP's displacement due to the ion concentration gradient.
Taking into account the temperature dependence of such
previously unknown parameters is a relevant step to describe
the temperature dependence of the NP's Soret coefficient.},
cin = {ICS-3},
ddc = {530},
cid = {I:(DE-Juel1)ICS-3-20110106},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551)},
pid = {G:(DE-HGF)POF3-551},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000454428800014},
doi = {10.1103/PhysRevE.98.062615},
url = {https://juser.fz-juelich.de/record/859035},
}