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@ARTICLE{Bocquet:859057,
      author       = {Bocquet, F. C. and Giovanelli, L. and Ksari, Y. and
                      Ovramenko, T. and Mayne, A. J. and Dujardin, G. and
                      Spillebout, F. and Sonnet, P. and Bondino, F. and Magnano,
                      E. and Themlin, J-M},
      title        = {{P}eculiar covalent bonding of {C} 60 /6 {H}
                      -{S}i{C}(0 0 0 1)-(3 × 3) probed by photoelectron
                      spectroscopy},
      journal      = {Journal of physics / Condensed matter Condensed matter},
      volume       = {30},
      number       = {50},
      issn         = {1361-648X},
      address      = {Bristol},
      publisher    = {IOP Publ.80390},
      reportid     = {FZJ-2019-00008},
      pages        = {505002 -},
      year         = {2018},
      abstract     = {High resolution photoemission with synchrotron radiation
                      was used to study the interfaceformation of a thin layer of
                      C60 on 6H-SiC(0 0 0 1)-(3 × 3), characterized by
                      protrudingSi-tetramers. The results show that C60 is
                      chemisorbed by orbital hybridization between
                      thehighest-occupied molecular orbital (HOMO) and the pz
                      orbital of Si adatom at the apex ofthe tetramers. The
                      covalent nature of the bonding was inferred from core level
                      as well asvalence band spectra. The Si 2p spectra reveal
                      that a large fraction (at least $45\%)$ of the Siadatoms
                      remain unbound despite the reactive character of the
                      associated dangling bonds.This is consistent with a model in
                      which each C60 is attached to the substrate through a
                      singlecovalent C60–Si bond. A binding energy shift of the
                      core levels associated with sub-surface Sior C atoms
                      indicates a decrease of the SiC band bending caused by a
                      charge transfer from theC60 molecules to the substrate via
                      the formation of donor-like interface states.},
      cin          = {PGI-3},
      ddc          = {530},
      cid          = {I:(DE-Juel1)PGI-3-20110106},
      pnm          = {523 - Controlling Configuration-Based Phenomena (POF3-523)},
      pid          = {G:(DE-HGF)POF3-523},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:30468155},
      UT           = {WOS:000451067900001},
      doi          = {10.1088/1361-648X/aaed1a},
      url          = {https://juser.fz-juelich.de/record/859057},
}