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000859104 1001_ $$00000-0002-9994-8461$$aFernandez-Castanon, J.$$b0$$eCorresponding author
000859104 245__ $$aAll-DNA System Close to the Percolation Threshold
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000859104 520__ $$aWe characterize via small-angle neutron scattering the structural properties of a mixture of all-DNA particles with functionalities 4 (A) and 2 (B) constrained by design to reside close to the percolation threshold. DNA base sequences are selected such that A particles can only bind with B ones and that at the studied temperature (10 °C) all AB bonds are formed and long-lived, originating highly polydisperse persistent equilibrium clusters. The concentration dependence of the scattered intensity and its wavevector dependence is exploited to determine the fractal dimension and the size distribution of the clusters, which are found to be consistent with the critical exponents of the 3-D percolation universality class. The value of DNA nanoparticles as nanometric patchy colloids with well-defined functionality, bonding selectivity, and exquisite control of the interaction strength is demonstrated.
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000859104 7001_ $$00000-0001-5160-6844$$aComez, L.$$b2
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