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@ARTICLE{Winter:859107,
      author       = {Winter, Martin and Barnett, Brian and Xu, Kang},
      title        = {{B}efore {L}i {I}on {B}atteries},
      journal      = {Chemical reviews},
      volume       = {118},
      number       = {23},
      issn         = {1520-6890},
      address      = {Washington, DC},
      publisher    = {ACS Publ.},
      reportid     = {FZJ-2019-00051},
      pages        = {11433 - 11456},
      year         = {2018},
      abstract     = {This Review covers a sequence of key discoveries and
                      technical achievements that eventually led to the birth of
                      the lithium-ion battery. In doing so, it not only sheds
                      light on the history with the advantage of contemporary
                      hindsight but also provides insight and inspiration to aid
                      in the ongoing quest for better batteries of the future. A
                      detailed retrospective on ingenious designs, accidental
                      discoveries, intentional breakthroughs, and deceiving
                      misconceptions is given: from the discovery of the element
                      lithium to its electrochemical synthesis; from intercalation
                      host material development to the concept of
                      dual-intercalation electrodes; and from the misunderstanding
                      of intercalation behavior into graphite to the comprehension
                      of interphases. The onerous demands of bringing all critical
                      components (anode, cathode, electrolyte, solid-electrolyte
                      interphases), each of which possess unique chemistries, into
                      a sophisticated electrochemical device reveal that the
                      challenge of interfacing these originally incongruent
                      components often outweighs the individual merits and limits
                      in their own properties. These important lessons are likely
                      to remain true for the more aggressive battery chemistries
                      of future generations, ranging from a revisited Li-metal
                      anode, to conversion-reaction type chemistries such as
                      Li/sulfur, Li/oxygen, and metal fluorides, and to bivalent
                      cation intercalations.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:30500179},
      UT           = {WOS:000453488700005},
      doi          = {10.1021/acs.chemrev.8b00422},
      url          = {https://juser.fz-juelich.de/record/859107},
}