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| Home > Publications database > Towards the development of materials for chemically stable carbonate-ceramic membranes to be used for CO2 separation in water-gas-shift reactorsek > print |
| Home > Publications database > Towards the development of materials for chemically stable carbonate-ceramic membranes to be used for CO2 separation in water-gas-shift reactorsek > print |
| 001 | 859216 | ||
| 005 | 20240709094448.0 | ||
| 024 | 7 | _ | |a 10.1016/j.seppur.2019.01.020 |2 doi |
| 024 | 7 | _ | |a 1383-5866 |2 ISSN |
| 024 | 7 | _ | |a 1873-3794 |2 ISSN |
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| 100 | 1 | _ | |a Gude, Ursula |0 P:(DE-Juel1)171634 |b 0 |e Corresponding author |u fzj |
| 245 | _ | _ | |a Towards the development of materials for chemically stable carbonate-ceramic membranes to be used for CO2 separation in water-gas-shift reactorsek |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2019 |b Elsevier Science |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1547825827_26450 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a Synthesis gas with a CO/H2 ratio suitable for production of energy carriers, e.g. hydrogen, methanol, and gasoline, can be produced by gasification of solid fuels with subsequent water-gas-shift (WGS) reaction. The separation of CO2 using conventional absorption processes leads to high efficiency losses. In contrast, a membrane reactor containing a catalyst provides the opportunity for significantly reduced efficiency losses.The present work aims at developing a chemically stable membrane for separation of carbon dioxide in gasification atmosphere. The desired membrane consists of two phases, a porous ceramic oxygen ion conductor filled with molten carbonate. Both phases need to be stable under the relevant process conditions, i.e. syngas at up to 800 °C, and compatible with each other and the water gas shift catalyst. The potential oxygen ion conductor materials, e.g. cerium gadolinium oxide (Ce0.8Gd0.2O2-δ) and cerium samarium oxide (Ce0.8Sm0.2O2-δ), which are known from literature to be compatible with alkali carbonate melts, were exposed to different gasification-relevant gas atmospheres at 600–900 °C and subsequently investigated regarding chemical reactions. Furthermore thermodynamic properties of alkali and alkaline earth carbonate systems were studied to identify a mixture with suitable melting behavior and high chemical stability as well as low volatility under relevant syngas conditions. |
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| 700 | 1 | _ | |a Baumann, Stefan |0 P:(DE-Juel1)129587 |b 1 |
| 700 | 1 | _ | |a Meulenberg, Wilhelm Albert |0 P:(DE-Juel1)129637 |b 2 |u fzj |
| 700 | 1 | _ | |a Müller, Michael |0 P:(DE-Juel1)129765 |b 3 |u fzj |
| 773 | _ | _ | |a 10.1016/j.seppur.2019.01.020 |g p. S1383586618326364 |0 PERI:(DE-600)2022535-0 |p 378-383 |t Separation and purification technology |v 215 |y 2019 |x 1383-5866 |
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