% IMPORTANT: The following is UTF-8 encoded. This means that in the presence % of non-ASCII characters, it will not work with BibTeX 0.99 or older. % Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or % “biber”. @ARTICLE{Alahmari:859588, author = {Alahmari, Fatimah and Davaasuren, Bambar and Emwas, Abdul-Hamid and Rothenberger, Alexander}, title = {{T}hioaluminogermanate {M}({A}l{S}2)({G}e{S}2)4 ({M} = {N}a, {A}g, {C}u): {S}ynthesis, {C}rystal {S}tructures, {C}haracterization, {I}on-{E}xchange and {S}olid-{S}tate 27{A}l and 23{N}a {NMR} {S}pectroscopy}, journal = {Inorganic chemistry}, volume = {57}, number = {7}, issn = {1520-510X}, address = {Washington, DC}, publisher = {American Chemical Society}, reportid = {FZJ-2019-00437}, pages = {3713 - 3719}, year = {2018}, abstract = {The new thioaluminogermanate Na(AlS2)(GeS2)4 (1) was successfully synthesized by a direct combination reaction. The compound crystallizes in the monoclinic space group P21/n (no. 14) with unit cell parameters a = 6.803(3) Å, b = 38.207(2) Å, c = 6.947(4) Å, and β = 119.17(3)°. The crystal structure is composed of a [(AlS2)(GeS2)4]− 3D polyanionic network, in which Al and Ge atoms share the atomic positions and Na cations occupy the channels and voids formed by the connection of (Ge/Al)S4 tetrahedra. The title compound shows a cation-exchange property with monovalent Ag+ and Cu+ ions at room temperature in solvent media, resulting in the formation of the isostructural compounds Ag(AlS2)(GeS2)4 (2) and Cu(AlS2)(GeS2)4 (3), respectively. The ion-exchange products Ag(AlS2)(GeS2)4 (2) and Cu(AlS2)(GeS2)4 (3) show higher air stability and narrower bandgap energies compared to those of the parent compound Na(AlS2)(GeS2)4 (1).}, cin = {IEK-1}, ddc = {540}, cid = {I:(DE-Juel1)IEK-1-20101013}, pnm = {131 - Electrochemical Storage (POF3-131)}, pid = {G:(DE-HGF)POF3-131}, typ = {PUB:(DE-HGF)16}, pubmed = {pmid:29537828}, UT = {WOS:000429283200028}, doi = {10.1021/acs.inorgchem.7b02980}, url = {https://juser.fz-juelich.de/record/859588}, }