Home > Publications database > Depth-resolved charge reconstruction at the LaNi O 3 / CaMn O 3 interface > print |
001 | 859719 | ||
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024 | 7 | _ | |a 10.1103/PhysRevB.98.155103 |2 doi |
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024 | 7 | _ | |a 2469-9969 |2 ISSN |
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100 | 1 | _ | |a Chandrasena, R. U. |0 P:(DE-HGF)0 |b 0 |
245 | _ | _ | |a Depth-resolved charge reconstruction at the LaNi O 3 / CaMn O 3 interface |
260 | _ | _ | |a Woodbury, NY |c 2018 |b Inst. |
336 | 7 | _ | |a article |2 DRIVER |
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520 | _ | _ | |a Rational design of low-dimensional electronic phenomena at oxide interfaces is currently considered to be one of the most promising schemes for realizing new energy-efficient logic and memory devices. An atomically abrupt interface between paramagnetic LaNiO3 and antiferromagnetic CaMnO3 exhibits interfacial ferromagnetism, which can be tuned via a thickness-dependent metal-insulator transition in LaNiO3. Once fully understood, such emergent functionality could turn this archetypal Mott-interface system into a key building block for the above-mentioned future devices. Here, we use depth-resolved standing-wave photoemission spectroscopy in conjunction with scanning transmission electron microscopy and x-ray absorption spectroscopy, to demonstrate a depth-dependent charge reconstruction at the LaNiO3/CaMnO3 interface. Our measurements reveal an increased concentration of Mn3+ and Ni2+ cations at the interface, which create an electronic environment favorable for the emergence of interfacial ferromagnetism mediated via the Mn4+−Mn3+ ferromagnetic double exchange and Ni2+−O−Mn4+ superexchange mechanisms. Our findings suggest a strategy for designing functional Mott oxide heterostructures by tuning the interfacial cation characteristics via controlled manipulation of thickness, strain, and ionic defect states. |
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542 | _ | _ | |i 2018-10-01 |2 Crossref |u https://link.aps.org/licenses/aps-default-license |
542 | _ | _ | |i 2019-10-01 |2 Crossref |u https://link.aps.org/licenses/aps-default-accepted-manuscript-license |
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700 | 1 | _ | |a Yang, W. |0 P:(DE-Juel1)176123 |b 2 |e Editor |
700 | 1 | _ | |a Arab, Arian |0 P:(DE-HGF)0 |b 3 |
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700 | 1 | _ | |a Suzuki, Y. |0 P:(DE-HGF)0 |b 15 |
700 | 1 | _ | |a Gray, A. X. |0 P:(DE-HGF)0 |b 16 |e Corresponding author |
773 | 1 | 8 | |a 10.1103/physrevb.98.155103 |b American Physical Society (APS) |d 2018-10-01 |n 15 |p 155103 |3 journal-article |2 Crossref |t Physical Review B |v 98 |y 2018 |x 2469-9950 |
773 | _ | _ | |a 10.1103/PhysRevB.98.155103 |g Vol. 98, no. 15, p. 155103 |0 PERI:(DE-600)2844160-6 |n 15 |p 155103 |t Physical review / B |v 98 |y 2018 |x 2469-9950 |
856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/859719/files/PhysRevB.98.155103.pdf |
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