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@ARTICLE{Simonenko:859746,
author = {Simonenko, Elizaveta P. and Simonenko, Nikolay P. and
Kopitsa, Gennady P. and Mokrushin, Artem S. and Khamova,
Tamara V. and Sizova, Svetlana V. and Khaddazh, Mishal and
Tsvigun, Natalia V. and Pipich, Vitaliy and Gorshkova, Yulia
E. and Sevastyanov, Vladimir G. and Kuznetsov, Nikolay T.},
title = {{A} sol-gel synthesis and gas-sensing properties of finely
dispersed {Z}r{T}i{O}4},
journal = {Materials chemistry and physics},
volume = {225},
issn = {0254-0584},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2019-00583},
pages = {347 - 357},
year = {2019},
abstract = {The transparent titanium-zirconium-containing gel was
obtained using heteroligand coordination compounds (namely,
alkoxoacetylacetonates) as the precursors. The
high-dispersive system “ZrTiO4 – carbon”, formed after
drying of such gel and carbonization of the obtained
xerogel, was used to study the evolution of microstructure
for the product (ZrTiO4) during thermal treatment in air for
1 h in the temperature range from 500 °C to 1000°С. It
was stated that the formation of crystalline phase occurred
in the narrow range 690-730°С. The thermal treatment at
500 °C and 600°С allowed obtaining micro- and mesoporous
X-ray amorphous products of the composition ZrTiO4, with the
specific surface area falling in the range 82–150m2/g. At
the higher temperatures the single-phase nanocrystalline
powder was prepared (the specific surface area amounted to
2.5–15m2/g). Particle coarsening took place more
extensively at temperatures ≥700°С was shown. For the
ZrTiO4 nanopowder crystallized under the mildest conditions
at the temperature of 700 °C, chemoresistive gas-sensitive
properties were studied for the first time. The material
showed a high reproducible response at $1–20\%$ O2 and
200–10,000 ppm H2 at a relatively low detection operating
temperature of 450 °C.},
cin = {JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6G15 - FRM II / MLZ (POF3-6G15)},
pid = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
experiment = {EXP:(DE-MLZ)KWS3-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000463847900047},
doi = {10.1016/j.matchemphys.2018.12.102},
url = {https://juser.fz-juelich.de/record/859746},
}