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@ARTICLE{Weidener:859867,
      author       = {Weidener, Dennis and Klose, Holger and Leitner, Walter and
                      Schurr, Ulrich and Usadel, Björn and DomínguezdeMaría,
                      Pablo and Grande, Philipp},
      title        = {{O}ne-{S}tep {L}ignocellulose {F}ractionation by using
                      2,5-{F}urandicarboxylic {A}cid as a {B}iogenic and
                      {R}ecyclable {C}atalyst},
      journal      = {ChemSusChem},
      volume       = {11},
      number       = {13},
      issn         = {1864-5631},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2019-00689},
      pages        = {2051 - 2056},
      year         = {2018},
      abstract     = {To develop novel biorefinery concepts, the use of
                      bio‐based catalysts and solvents must be aligned with the
                      principles of green chemistry. In this context, biogenic
                      2,5‐furandicarboxylic acid (FDCA) is a very promising yet
                      underused molecule with high potential for application as an
                      acid catalyst, combining feasibility and sustainability with
                      efficient and straightforward recovery. In this study, FDCA
                      was evaluated as a catalyst in the recently developed
                      OrganoCat pretreatment, a biphasic lignocellulose
                      fractionation system. The catalyst was investigated for the
                      efficient fractionation of the three main
                      components—lignin, cellulose and noncellulosic
                      sugars—with particular focus on the lignin quality, on the
                      effect on enzymatic hydrolysis of the cellulosic residue,
                      and on the noncellulosic sugar extraction. To address
                      recovery of FDCA from the OrganoCat system, a method was
                      developed, leading to the recovery of $>97 \%$ of FDCA
                      with a spectroscopic purity of $>99 \%,$ maintaining full
                      activity in consecutive runs},
      cin          = {IBG-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IBG-2-20101118},
      pnm          = {582 - Plant Science (POF3-582)},
      pid          = {G:(DE-HGF)POF3-582},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:29791080},
      UT           = {WOS:000438198400006},
      doi          = {10.1002/cssc.201800653},
      url          = {https://juser.fz-juelich.de/record/859867},
}