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000860153 1001_ $$0P:(DE-Juel1)161444$$aLobe, Sandra$$b0$$eCorresponding author
000860153 245__ $$aChallenges regarding thin film deposition of garnet electrolytes for all-solid-state lithium batteries with high energy density
000860153 260__ $$aHeidelberg$$bSpringer$$c2018
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000860153 520__ $$aIn this work, we studied the deposition of garnet electrolyte thin films in order to realize an all-solid-state battery with high energy density. Therefore, in a first step we investigated the stability of the garnet Li5La3Ta2O12 with the spinel LiCoMnO4 in order to determine the temperature window for a successful thin film deposition on high-voltage spinels. A mixture of both materials showed a thermal stability up to 600 °C, so that all-solid-state batteries could be realized when the electrolyte is applied at a low deposition temperature. The second part of the work was the thin film deposition of Li5La3Ta2O12 by a sputter deposition process. When a stoichiometric Li5La3Ta2O12 sputter target was used, the surface of the target showed a depletion of lithium after several depositions, which leads to decreasing Li content in the thin films. In order to compensate the lithium loss we enriched the target with LiOH∙H
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000860153 7001_ $$0P:(DE-Juel1)165951$$aWindmüller, A.$$b2$$ufzj
000860153 7001_ $$0P:(DE-Juel1)156244$$aTsai, C.-L.$$b3$$ufzj
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000860153 7001_ $$0P:(DE-Juel1)161591$$aGuillon, O.$$b6$$ufzj
000860153 773__ $$0PERI:(DE-600)2226746-3$$a10.1007/s11581-018-2594-3$$gVol. 24, no. 8, p. 2199 - 2208$$n8$$p2199 - 2208$$tIonics$$v24$$x1862-0760$$y2018
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