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@ARTICLE{Lobe:860153,
      author       = {Lobe, Sandra and Dellen, C. and Windmüller, A. and Tsai,
                      C.-L. and Vondahlen, F. and Uhlenbruck, S. and Guillon, O.},
      title        = {{C}hallenges regarding thin film deposition of garnet
                      electrolytes for all-solid-state lithium batteries with high
                      energy density},
      journal      = {Ionics},
      volume       = {24},
      number       = {8},
      issn         = {1862-0760},
      address      = {Heidelberg},
      publisher    = {Springer},
      reportid     = {FZJ-2019-00939},
      pages        = {2199 - 2208},
      year         = {2018},
      abstract     = {In this work, we studied the deposition of garnet
                      electrolyte thin films in order to realize an
                      all-solid-state battery with high energy density. Therefore,
                      in a first step we investigated the stability of the garnet
                      Li5La3Ta2O12 with the spinel LiCoMnO4 in order to determine
                      the temperature window for a successful thin film deposition
                      on high-voltage spinels. A mixture of both materials showed
                      a thermal stability up to 600 °C, so that all-solid-state
                      batteries could be realized when the electrolyte is applied
                      at a low deposition temperature. The second part of the work
                      was the thin film deposition of Li5La3Ta2O12 by a sputter
                      deposition process. When a stoichiometric Li5La3Ta2O12
                      sputter target was used, the surface of the target showed a
                      depletion of lithium after several depositions, which leads
                      to decreasing Li content in the thin films. In order to
                      compensate the lithium loss we enriched the target with
                      LiOH∙H},
      cin          = {IEK-1},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {131 - Electrochemical Storage (POF3-131) / BMBF-03SF0477A -
                      DESIREE : Defektspinelle als Hochenergie- und
                      Hochleistungsmaterialien zur elektrochemischen
                      Energiespeicherung, Teilprojekte:
                      Partikelmikrostrukturierung und Modellsysteme,
                      Makroskopische und atomistische Analyse von
                      elektrochemischen Vorgängen (BMBF-03SF0477A)},
      pid          = {G:(DE-HGF)POF3-131 / G:(DE-82)BMBF-03SF0477A},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000437826300004},
      doi          = {10.1007/s11581-018-2594-3},
      url          = {https://juser.fz-juelich.de/record/860153},
}