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| Hauptseite > Publikationsdatenbank > Stabilizing the Interface of NASICON Solid Electrolyte against Li Metal with Atomic Layer Deposition > print |
| Hauptseite > Publikationsdatenbank > Stabilizing the Interface of NASICON Solid Electrolyte against Li Metal with Atomic Layer Deposition > print |
| 001 | 860249 | ||
| 005 | 20240711085552.0 | ||
| 024 | 7 | _ | |a 10.1021/acsami.8b06366 |2 doi |
| 024 | 7 | _ | |a 1944-8244 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2019-01033 |
| 082 | _ | _ | |a 600 |
| 100 | 1 | _ | |a Liu, Yulong |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Stabilizing the Interface of NASICON Solid Electrolyte against Li Metal with Atomic Layer Deposition |
| 260 | _ | _ | |a Washington, DC |c 2018 |b Soc. |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Solid-state batteries have been considered as one of the most promising next-generation energy storage systems because of their high safety and energy density. Solid-state electrolytes are the key component of the solid-state battery, which exhibit high ionic conductivity, good chemical stability, and wide electrochemical windows. LATP [Li1.3Al0.3Ti1.7 (PO4)3] solid electrolyte has been widely investigated for its high ionic conductivity. Nevertheless, the chemical instability of LATP against Li metal has hindered its application in solid-state batteries. Here, we propose that atomic layer deposition (ALD) coating on LATP surfaces is able to stabilize the LATP/Li interface by reducing the side reactions. In comparison with bare LATP, the Al2O3-coated LATP by ALD exhibits a stable cycling behavior with smaller voltage hysteresis for 600 h, as well as small resistance. More importantly, on the basis of advanced characterizations such as high-resolution transmission electron spectroscope-electron energy loss spectroscopy, the lithium penetration into the LATP bulk and Ti4+ reduction are significantly limited. The results suggest that ALD is very effective in improving solid-state electrolyte/electrode interface stability. |
| 536 | _ | _ | |a 131 - Electrochemical Storage (POF3-131) |0 G:(DE-HGF)POF3-131 |c POF3-131 |f POF III |x 0 |
| 588 | _ | _ | |a Dataset connected to CrossRef |
| 700 | 1 | _ | |a Sun, Qian |0 0000-0001-5399-1440 |b 1 |
| 700 | 1 | _ | |a Zhao, Yang |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Wang, Biqiong |0 0000-0002-3903-8634 |b 3 |
| 700 | 1 | _ | |a Kaghazchi, Payam |0 P:(DE-Juel1)174502 |b 4 |e Corresponding author |
| 700 | 1 | _ | |a Adair, Keegan R. |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Li, Ruying |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Zhang, Cheng |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Liu, Jingru |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Kuo, Liang-Yin |0 P:(DE-Juel1)177014 |b 9 |
| 700 | 1 | _ | |a Hu, Yongfeng |0 P:(DE-HGF)0 |b 10 |
| 700 | 1 | _ | |a Sham, Tsun-Kong |0 P:(DE-HGF)0 |b 11 |
| 700 | 1 | _ | |a Zhang, Li |0 P:(DE-HGF)0 |b 12 |
| 700 | 1 | _ | |a Yang, Rong |0 P:(DE-HGF)0 |b 13 |
| 700 | 1 | _ | |a Lu, Shigang |0 P:(DE-HGF)0 |b 14 |
| 700 | 1 | _ | |a Song, Xiping |0 P:(DE-HGF)0 |b 15 |
| 700 | 1 | _ | |a Sun, Xueliang |0 0000-0003-2881-8237 |b 16 |
| 773 | _ | _ | |a 10.1021/acsami.8b06366 |g Vol. 10, no. 37, p. 31240 - 31248 |0 PERI:(DE-600)2467494-1 |n 37 |p 31240 - 31248 |t ACS applied materials & interfaces |v 10 |y 2018 |x 1944-8252 |
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