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000860279 1001_ $$0P:(DE-HGF)0$$aJing, Hong-Mei$$b0
000860279 245__ $$aFormation of Ruddlesden–Popper Faults and Their Effect on the Magnetic Properties in Pr 0.5 Sr 0.5 CoO 3 Thin Films
000860279 260__ $$aWashington, DC$$bSoc.$$c2018
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000860279 520__ $$aEpitaxial Pr0.5Sr0.5CoO3 thin films have been grown on single-crystalline (La0.289Sr0.712)(Al0.633Ta0.356)O3(001) substrates by the pulsed laser deposition technique. The magnetic properties and microstructure of these films are investigated. It is found that Ruddlesden–Popper faults (RP faults) can be introduced in the films by changing the laser repetition rate. The segregation of Pr at the RP faults is characterized by atomic-resolution chemical mapping. The formation of the RP faults not only contributes to the epitaxial strain relaxation but also significantly decreases the ferromagnetic long-range order of the films, resulting in lower magnetizations than those of the fault-free films. Our results provide a strategy for tuning the magnetic properties of cobalt-based perovskite films by modifying the microstructure through the film growth process.
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000860279 7001_ $$0P:(DE-HGF)0$$aCheng, Sheng$$b1
000860279 7001_ $$00000-0001-5711-850X$$aMi, Shao-Bo$$b2$$eCorresponding author
000860279 7001_ $$0P:(DE-Juel1)161232$$aLu, Lu$$b3
000860279 7001_ $$00000-0002-4392-9659$$aLiu, Ming$$b4
000860279 7001_ $$0P:(DE-HGF)0$$aCheng, Shao-Dong$$b5
000860279 7001_ $$0P:(DE-Juel1)130736$$aJia, Chun-Lin$$b6
000860279 773__ $$0PERI:(DE-600)2467494-1$$a10.1021/acsami.7b16341$$gVol. 10, no. 1, p. 1428 - 1433$$n1$$p1428 - 1433$$tACS applied materials & interfaces$$v10$$x1944-8252$$y2018
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