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@ARTICLE{Wang:860295,
author = {Wang, Jiangjing and Ronneberger, Ider and Zhou, Ling and
Lu, Lu and Deringer, Volker L. and Zhang, Baiyu and Tian,
Lin and Du, Hongchu and Jia, Chunlin and Qian, Xiaofeng and
Wuttig, Matthias and Mazzarello, Riccardo and Zhang, Wei},
title = {{U}nconventional two-dimensional germanium dichalcogenides},
journal = {Nanoscale},
volume = {10},
number = {16},
issn = {2040-3372},
address = {Cambridge},
publisher = {RSC Publ.},
reportid = {FZJ-2019-01070},
pages = {7363 - 7368},
year = {2018},
abstract = {The recently discovered two-dimensional (2D) group IV
chalcogenides attract much attention owing to their novel
electronic and photonic properties. All the reported
materials of this class favor (distorted) octahedral
coordination via p bonding; by contrast, in the
dichalcogenides where the bonding tendency approaches sp3,
no corresponding 2D phase has been realized so far. Here, by
engineering the composition of a chalcogenide
heterostructure, the hitherto elusive GeTe2 is
experimentally observed in a confined 2D environment.
Density functional theory simulations predict the existence
of a freestanding monolayer of octahedrally coordinated
GeTe2 under tensile strain, and the existence of GeSe2 and
GeS2 in the same form under equilibrium conditions. These 2D
germanium dichalcogenides are either metallic or narrow gap
semiconducting, and may lead to new applications in
nanoscale electronics.},
cin = {ER-C-1 / JARA-HPC / JARA-FIT},
ddc = {600},
cid = {I:(DE-Juel1)ER-C-1-20170209 / $I:(DE-82)080012_20140620$ /
$I:(DE-82)080009_20140620$},
pnm = {143 - Controlling Configuration-Based Phenomena (POF3-143)
/ Ab initio study of interfacial phase-change materials and
thin chalcogenides $(jara0150_20160501)$},
pid = {G:(DE-HGF)POF3-143 / $G:(DE-Juel1)jara0150_20160501$},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:29637969},
UT = {WOS:000431030000005},
doi = {10.1039/C8NR01747F},
url = {https://juser.fz-juelich.de/record/860295},
}