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@ARTICLE{Haque:860635,
author = {Haque, Md Azimul and Gandi, Appala Naidu and Mohanraman,
Rajeshkumar and Weng, Yakui and Davaasuren, Bambar and
Emwas, Abdul‐Hamid and Combe, Craig and Baran, Derya and
Rothenberger, Alexander and Schwingenschlögl, Udo and
Alshareef, Husam N. and Dong, Shuai and Wu, Tom},
title = {{A} 0{D} {L}ead‐{F}ree {H}ybrid {C}rystal with {U}ltralow
{T}hermal {C}onductivity},
journal = {Advanced functional materials},
volume = {29},
number = {13},
issn = {1616-3028},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2019-01308},
pages = {1809166},
year = {2019},
abstract = {Organic–inorganic hybrid materials are of significant
interest owing to their diverse applications ranging from
photovoltaics and electronics to catalysis. Control over the
organic and inorganic components offers flexibility through
tuning their chemical and physical properties. Herein, it is
reported that a new organic–inorganic hybrid,
[Mn(C2H6OS)6]I4, with linear tetraiodide anions exhibit an
ultralow thermal conductivity of 0.15 ± 0.01 W m−1 K−1
at room temperature, which is among the lowest values
reported for organic–inorganic hybrid materials.
Interestingly, the hybrid compound has a unique 0D
structure, which extends into 3D supramolecular frameworks
through nonclassical hydrogen bonding. Phonon band structure
calculations reveal that low group velocities and
localization of vibrational energy underlie the observed
ultralow thermal conductivity, which could serve as a
general principle to design novel thermal management
materials.},
cin = {IEK-1},
ddc = {530},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000463732400025},
doi = {10.1002/adfm.201809166},
url = {https://juser.fz-juelich.de/record/860635},
}