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@ARTICLE{Tsai:861198,
      author       = {Tsai, Chih-Long and Ma, Qianli and Dellen, Christian and
                      Lobe, Sandra and Vondahlen, Frank and Windmüller, Anna and
                      Grüner, Daniel and Zheng, Hao and Uhlenbruck, Sven and
                      Finsterbusch, Martin and Tietz, Frank and
                      Fattakhova-Rohlfing, Dina and Buchkremer, Hans Peter and
                      Guillon, Olivier},
      title        = {{A} garnet structure-based all-solid-state {L}i battery
                      without interface modification: resolving incompatibility
                      issues on positive electrodes},
      journal      = {Sustainable energy $\&$ fuels},
      volume       = {3},
      number       = {1},
      issn         = {2398-4902},
      address      = {Cambridge},
      publisher    = {Royal Society of Chemistry},
      reportid     = {FZJ-2019-01730},
      pages        = {280 - 291},
      year         = {2019},
      abstract     = {The development of high-performance Li7La3Zr2O12
                      (LLZO)-based all-solid-state lithium batteries (SSLB)
                      isusually hampered by highly resistive interfaces due to the
                      need for sintering at elevated temperatures toform ionic
                      diffusion paths through the grains. Many strategies have
                      been proposed to solve the problembut the achievements have
                      been limited. Herein, a new design principle is introduced,
                      based on cosinteringcrystalline LCO and Ta-substituted LLZO
                      instead of using the more reactive Li–Co–Oprecursors and
                      Al-substituted LLZO, which allows the fabrication of high
                      specific areal density and lowcell area resistance without
                      the interface modification of LLZO-based SSLB. Detailed
                      studies usingmicro-Raman and EDS mapping revealed that the
                      well-sintered interfaces are free from detrimentalsecondary
                      phases. To demonstrate that a true bulk-type SSLB can be
                      constructed by this straightforwardstrategy, the material
                      loading for a composite positive electrode was increased to
                      about 10 times that inprevious reports, which resulted in a
                      high areal capacity of 1.63 mA h cm2 (i.e. 110 mA h g1)
                      whendischarged with a current density of 50 mA cm2. It also
                      allows one to discharge the fabricated SSLB ata very high
                      current density of 500 mA cm2 at 50 C due to the minimized
                      cell areal resistance. The newfabrication strategy for the
                      LLZO-based SSLB paves the way for achieving SSLB with high
                      safety andenergy density.},
      cin          = {IEK-1 / IEK-2},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-2-20101013},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000453816900019},
      doi          = {10.1039/C8SE00436F},
      url          = {https://juser.fz-juelich.de/record/861198},
}