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@ARTICLE{Du:861799,
author = {Du, Nan and Manjunath, Niveditha and Li, Yuan and Menzel,
Stephan and Waser, R. and Linn, Eike and You, Tiangui and
Bürger, Danilo and Skorupa, Ilona and Walczyk, Damian and
Walczyk, Christian and Schmidt, Oliver G. and Schmidt,
Heidemarie},
title = {{F}ield-{D}riven {H}opping {T}ransport of {O}xygen
{V}acancies in {M}emristive {O}xide {S}witches with
{I}nterface-{M}ediated {R}esistive {S}witching},
journal = {Physical review applied},
volume = {10},
number = {5},
issn = {2331-7019},
address = {College Park, Md. [u.a.]},
publisher = {American Physical Society},
reportid = {FZJ-2019-02227},
pages = {054025},
year = {2018},
abstract = {We investigate the hopping transport of positively charged
mobile oxygen vacancies V+o in electroforming-free bipolar
memristive BiFeO3 switches by conducting impedance
spectroscopy and quasistatic state-test measurements. We
demonstrate that BiFeO3 switches with mobile oxygen
vacancies (V+o) and fixed substitutional Ti4+ donors on Fe3+
lattice sites close to the bottom electrode have a
rectifying top electrode with an unflexible barrier height
and a rectifying and/or nonrectifying bottom electrode with
a flexible barrier height. The field-driven hopping
transport of the oxygen vacancies determines the
reconfiguration of the flexible barrier and the dynamics of
the resistive switching. Average activation energies of 0.53
eV for trapping and of 0.31 eV for the release of oxygen
vacancies by the Ti4+ donors during application of the SET
and RESET excitation pulses are extracted, respectively. The
larger activation energy during SET is experimentally
verified by impedance spectroscopy measurements and
evidences the local enhancement of the electrostatic
potential profile at the bottom electrode due to the Ti4+
donors on Fe3+ lattice sites.},
cin = {PGI-7 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$},
pnm = {521 - Controlling Electron Charge-Based Phenomena
(POF3-521)},
pid = {G:(DE-HGF)POF3-521},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000449792500003},
doi = {10.1103/PhysRevApplied.10.054025},
url = {https://juser.fz-juelich.de/record/861799},
}