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@ARTICLE{Scotti:861897,
      author       = {Scotti, A. and Bochenek, S. and Brugnoni, M. and
                      Fernandez-Rodriguez, M. A. and Schulte, M. F. and Houston,
                      J. E. and Gelissen, A. P. H. and Potemkin, I. I. and Isa, L.
                      and Richtering, W.},
      title        = {{E}xploring the colloid-to-polymer transition for ultra-low
                      crosslinked microgels from three to two dimensions},
      journal      = {Nature Communications},
      volume       = {10},
      number       = {1},
      issn         = {2041-1723},
      address      = {[London]},
      publisher    = {Nature Publishing Group UK},
      reportid     = {FZJ-2019-02318},
      pages        = {1418},
      year         = {2019},
      abstract     = {Microgels are solvent-swollen nano- and microparticles that
                      show prevalent colloidal-like behavior despite their
                      polymeric nature. Here we study ultra-low crosslinked
                      poly(N-isopropylacrylamide) microgels (ULC), which can
                      behave like colloids or flexible polymers depending on
                      dimensionality, compression or other external stimuli.
                      Small-angle neutron scattering shows that the structure of
                      the ULC microgels in bulk aqueous solution is characterized
                      by a density profile that decays smoothly from the center to
                      a fuzzy surface. Their phase behavior and rheological
                      properties are those of soft colloids. However, when these
                      microgels are confined at an oil-water interface, their
                      behavior resembles that of flexible macromolecules. Once
                      monolayers of ultra-low crosslinked microgels are
                      compressed, deposited on solid substrate and studied with
                      atomic-force microscopy, a concentration-dependent
                      topography is observed. Depending on the compression, these
                      microgels can behave as flexible polymers, covering the
                      substrate with a uniform film, or as colloidal microgels
                      leading to a monolayer of particles.},
      cin          = {JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
      ddc          = {500},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
                      / 6G15 - FRM II / MLZ (POF3-6G15)},
      pid          = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
      experiment   = {EXP:(DE-MLZ)KWS2-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:30926786},
      UT           = {WOS:000462721900017},
      doi          = {10.1038/s41467-019-09227-5},
      url          = {https://juser.fz-juelich.de/record/861897},
}