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024 7 _ |a 10.5194/acp-2018-1193
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100 1 _ |a Robrecht, Sabine
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245 _ _ |a Mechanism of ozone loss under enhanced water vapour conditions in the mid-latitude lower stratosphere in summer
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520 _ _ |a Water vapour convectively injected into the mid-latitude lowermost stratosphere could affect stratospheric ozone. The associated potential ozone loss process requires low temperatures and an elevated water vapour mixing ratio. An increase in sulphate aerosol surface area due to a volcanic eruption or geoengineering could increase the likelihood of occurrence of this process. However, the chemical mechanism of this ozone loss process has not yet been analysed in sufficient detail and its sensitivity to various conditions is not yet clear. Under conditions of climate change associated with an increase in greenhouse gases, both a stratospheric cooling and an increase in water vapour convectively injected into the stratosphere is expected. Understanding the influence of low temperatures, elevated water vapour and enhanced sulphate particles on this ozone loss mechanism is a key step in estimating the impact of climate change and potential sulphate geoengineering on mid-latitude ozone.
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700 1 _ |a Grooß, Jens-Uwe
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700 1 _ |a Rosenlof, Karen
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700 1 _ |a Thornberry, Troy
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700 1 _ |a Christensen, Lance
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700 1 _ |a Müller, Rolf
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Marc 21