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000862435 1001_ $$0P:(DE-Juel1)165914$$aPaulus, M. C.$$b0$$eCorresponding author
000862435 245__ $$aExperimental evidence for the relaxation coupling of all longitudinal 7Li magnetization orders in the superionic conductor Li10GeP2S12
000862435 260__ $$aAmsterdam [u.a.]$$bElsevier$$c2019
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000862435 520__ $$aThis contribution addresses the experimental proof of the relaxation coupling of the 7Li (I = 3/2) longitudinal magnetization orders in the solid-state electrolyte Li10GeP2S12 (LGPS). This effect was theoretically described by Korb and Petit in 1988 but has not yet been shown experimentally. In a 2D-T1/spin-alignment echo (SAE) experiment, the inverse Laplace transformation of the spectral component over two time dimensions revealed the asymmetric course of the spin-lattice relaxation following from the coupling of all longitudinal orders. These observations were supported by Multi-quantum-filter experiments and by simulations of the 2D-T1/SAE experiment with a lithium spin system. Since the asymmetric relaxation effects are directly dependent on the velocities and degrees of freedom of ion motion they could be used especially in fast Li-ion conductors as a separation tool for environments with different mobility processes.
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000862435 7001_ $$0P:(DE-Juel1)166099$$aPaulus, A.$$b1
000862435 7001_ $$0P:(DE-Juel1)168465$$aSchleker, Peter Philipp Maria$$b2$$ufzj
000862435 7001_ $$0P:(DE-Juel1)156296$$aJakes, P.$$b3
000862435 7001_ $$0P:(DE-Juel1)156123$$aEichel, R.-A.$$b4
000862435 7001_ $$0P:(DE-HGF)0$$aHeitjans, P.$$b5
000862435 7001_ $$0P:(DE-Juel1)162401$$aGranwehr, J.$$b6
000862435 773__ $$0PERI:(DE-600)1469665-4$$a10.1016/j.jmr.2019.04.006$$gVol. 303, p. 57 - 66$$p57 - 66$$tJournal of magnetic resonance$$v303$$x1090-7807$$y2019
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